Strongly confined Te quantum dots as building blocks for single photon sources
Tellurium is a heavy chemical element exhibiting chirality, anisotropy, and strong spin-orbit coupling; consequently, displaying a huge potential in quantum hardware technologies. In this article, tellurium quantum dots, with sizes around 19 ± 3 nm and energy bandgap around 2.4 eV, were successfully synthesized by pulsed laser ablation in liquids (PLAL). The synthesis was performed by using a nanosecond Nd:YAG laser emitting at 1064 nm and pulsing the laser beam at 1 kHz. Toluene (C 6 H 5 CH 3 ) was used as a solvent to avoid oxidation of the dots. Non-polarized and polarized Raman spectroscopy as well as X-Ray diffraction were performed on the dots to study their quantum confinement and anisotropy. Finally, strongly confined tellurium quantum dots were obtained; and, their properties underline their potential as quantum light sources.
Authors
- Grégory Guisbiers (ORCID: https://orcid.org/0000-0002-4615-6014)
- Julien Chaste (ORCID: https://orcid.org/0000-0001-8384-0133)
- Francisco Ruiz‐Zepeda (ORCID: https://orcid.org/0000-0002-2637-3433)
- Étienne Herth (ORCID: https://orcid.org/0000-0002-8321-5060)
- Thang B. Hoang (ORCID: https://orcid.org/0000-0001-6438-112X)
- Yagya Bahadur Woli (ORCID: https://orcid.org/0009-0005-2593-3776)
- R. Subedi (ORCID: https://orcid.org/0009-0002-8173-3179)
Institutions
- University of Arkansas at Little Rock (US)
- Université Paris-Saclay (FR)
- Centre de Nanosciences et de Nanotechnologies (FR)
- National Institute of Chemistry (SI)
- The University of Texas at San Antonio (US)
- University of Memphis (US)
- UCLouvain (BE)
Publication Details
- Journal
- Materials Today Quantum
- Published
- 2025-03-22
- DOI
- https://doi.org/10.1016/j.mtquan.2025.100034
- Citations
- 1
- Primary Topic
- Nonlinear Optical Materials Studies
- Type
- article
- Field-Weighted Citation Impact
- 0.67
Funders
- National Science Foundation
- Office for Science and Technology of the Embassy of France in the United States
- Agence Nationale de la Recherche
- European Research Council
- FP7 Ideas: European Research Council