A promising radiative cooling composite coatings based on hydromagnesite mineral for dual thermal management in human body and lithium-ion battery
• A hydromagnesite-based composite with selective optical response is reported. • Hydromagnesite-based composites can cool the human body and lithium-ion battery. • The radiative cooling textile cools simulated skin by 2 ∼ 10 ℃ below pristine textile. • The cooling ALF encapsulated lithium-ion battery reduces temperature by 8.1 °C. Radiative cooling emerges as an ideal solution to minimize the energy demand and environmental pollution associated with cooling applications. Herein, we report an industry-scalable radiative cooling technology capable of addressing the cooling demands from highly thermogenic sources by employing homemade hydromagnesite-based composites with excellent selective optical responses. First, relative to the pristine textile, the resulting radiative cooling textile modified by a hydromagnesite-polyacrylate (PA) composite coating possesses both high thermal emissivity (97.3 %) and solar reflectivity (90.2 %, and 95.5 % in the main solar waveband of 0.3–1.5 µm), which could cool the covered simulated skin by ∼ 2 and 10 ℃ in indoors and outdoors conditions, respectively. Second, when applied to lithium-ion battery, a temperature drop of 8.1 °C was realized when the battery was encapsulated by radiative cooling aluminum laminated film (ALF) modified with hydromagnesite-high-density polyethylene (HDPE) composites having an emissivity 92.6 %, thereby significantly improving its electrochemical behavior and operational performance, as well as safety by potentially avoiding the risk of a thermal runaway. The hydromagnesite-based composites also have good mechanical properties that are relevant to personal thermal management and lithium-ion battery cooling, enabling a substantial reduction in carbon emission and energy consumption associated with these cooling challenges.
Authors
- Leilei Du (ORCID: https://orcid.org/0000-0002-8522-9327)
- Mingwu Tan (ORCID: https://orcid.org/0000-0002-5099-7190)
- Renhong Li (ORCID: https://orcid.org/0000-0002-8327-5506)
- Jinhuan Zheng (ORCID: https://orcid.org/0000-0001-8903-110X)
- Bin Hu (ORCID: https://orcid.org/0000-0003-3143-746X)
- Zhengui Zhou
- Chenglong Wang (ORCID: https://orcid.org/0000-0001-5211-8041)
- Wen Liu (ORCID: https://orcid.org/0000-0002-1107-131X)
- Wenxing Chen (ORCID: https://orcid.org/0000-0002-4554-1455)
- Selvi Mushina
Institutions
- Agency for Science, Technology and Research (SG)
- Zhejiang Sci-Tech University (CN)
- Nanyang Technological University (SG)
- The Cambridge Centre for Advanced Research and Education in Singapore (SG)
- Wuhan National Laboratory for Optoelectronics (CN)
- Huazhong University of Science and Technology (CN)
Publication Details
- Journal
- Chemical Engineering Journal
- Published
- 2025-03-22
- DOI
- https://doi.org/10.1016/j.cej.2025.161730
- Citations
- 2
- Primary Topic
- Thermal Radiation and Cooling Technologies
- Type
- article
- Field-Weighted Citation Impact
- 1.91