Observation of Topological Spin Textures in Ferrimagnetic Mn<sub>2 − <i>x</i></sub>Zn<sub><i>x</i></sub>Sb

Ferrimagnets, which have both ferromagnetic and antiferromagnetic coupling, are attracting increased attention in the realm of spintronic devices due to advantages such as ultrafast dynamics and a suppressed skyrmion Hall effect. Thus, understanding the behavior of nontrivial spin textures in ferrimagnets is crucial; however, comprehensive reports on this topic remain limited. Here, the magnetic spin textures of ferrimagnetic Mn<sub>2 - x</sub>Zn<sub>x</sub>Sb (x = 0.85) is explored as a function of temperature and applied magnetic field. The spin textures can be tuned to a variety of states, including stripes, skyrmion bags, and a skyrmion lattice. Chiral Néel-type magnetic structures are visualized using Lorentz transmission electron microscopy. Mn(I) ions are slightly shifted toward the Sb sites, which may be due to a strong electrostatic interaction between Mn and Sb ions. This local structural distortion breaks the inversion symmetry and introduces an effective Dzyaloshinkii-Moriya interaction. This work thus provides a pathway to use doping and heterogeneity in a ferrimagnet to control and generate chiral nontrivial spin textures.

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Publication Details

Journal
Small
Published
2025-03-20
DOI
https://doi.org/10.1002/smll.202406299
Citations
2
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
2.49

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article

Observation of Topological Spin Textures in Ferrimagnetic Mn2 − xZnxSb

Stephan Rosenkranz, Charudatta Phatak, Hu Jin, Yuzi Liu et al.
2 citations
Small
Magnetic properties of thin films
2.49
article

Observation of Topological Spin Textures in Ferrimagnetic Mn2 − xZnxSb

Stephan Rosenkranz, Charudatta Phatak, Hu Jin, Yuzi Liu, Yue Li, A. K. Petford‐Long, Md Rafique Un Nabi, S. G. E. te Velthuis, Hyowon Park
article en
2 citations

Abstract

Ferrimagnets, which have both ferromagnetic and antiferromagnetic coupling, are attracting increased attention in the realm of spintronic devices due to advantages such as ultrafast dynamics and a suppressed skyrmion Hall effect. Thus, understanding the behavior of nontrivial spin textures in ferrimagnets is crucial; however, comprehensive reports on this topic remain limited. Here, the magnetic spin textures of ferrimagnetic Mn<sub>2 - x</sub>Zn<sub>x</sub>Sb (x = 0.85) is explored as a function of temperature and applied magnetic field. The spin textures can be tuned to a variety of states, including stripes, skyrmion bags, and a skyrmion lattice. Chiral Néel-type magnetic structures are visualized using Lorentz transmission electron microscopy. Mn(I) ions are slightly shifted toward the Sb sites, which may be due to a strong electrostatic interaction between Mn and Sb ions. This local structural distortion breaks the inversion symmetry and introduces an effective Dzyaloshinkii-Moriya interaction. This work thus provides a pathway to use doping and heterogeneity in a ferrimagnet to control and generate chiral nontrivial spin textures.

SmallVol. 21(17)
Northwestern University (US), Argonne National Laboratory (US), University of Illinois Chicago (US), University of Arkansas at Fayetteville (US)
National Science Foundation, U.S. Department of Energy, Office of Science, Argonne National Laboratory
Openalex Percentile: Top 13%
Magnetic properties of thin films
2.49
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