Self-assembling clusters of particles on a shrinking liquid surface

After rainfall, pine needles often float on the surface of small puddles. As the water evaporates, they self-assemble into distinct clusters. Motivated by this natural phenomenon, we experimentally investigate the dynamic evolution of synthetic particles as the liquid surface shrinks in area. Our experiments demonstrate the tendency of particles to aggregate, forming distinct clusters as the liquid boundary shrinks. We systematically examine the emergence of these clusters and explore how their sizes and numbers evolve with changes in the packing fraction. We also analyze particle rotation during the process and discuss the formation of the final configuration comprising clusters of various orientations. Complementary numerical simulations demonstrate qualitative agreement with our experimental findings. This study sheds additional light on the self-assembly of macroscopic particles in a dynamically evolving medium.

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Publication Details

Journal
Physical Review Research
Published
2025-03-20
DOI
https://doi.org/10.1103/physrevresearch.7.013293
Primary Topic
Pickering emulsions and particle stabilization
Type
article
Field-Weighted Citation Impact
0.00

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article

Self-assembling clusters of particles on a shrinking liquid surface

Duanduan Wan, Mark J. Bowick, Shuchen Zhang, Xin Li
Physical Review Research
Pickering emulsions and particle stabilization
article

Self-assembling clusters of particles on a shrinking liquid surface

Duanduan Wan, Mark J. Bowick, Shuchen Zhang, Xin Li
article en

Abstract

After rainfall, pine needles often float on the surface of small puddles. As the water evaporates, they self-assemble into distinct clusters. Motivated by this natural phenomenon, we experimentally investigate the dynamic evolution of synthetic particles as the liquid surface shrinks in area. Our experiments demonstrate the tendency of particles to aggregate, forming distinct clusters as the liquid boundary shrinks. We systematically examine the emergence of these clusters and explore how their sizes and numbers evolve with changes in the packing fraction. We also analyze particle rotation during the process and discuss the formation of the final configuration comprising clusters of various orientations. Complementary numerical simulations demonstrate qualitative agreement with our experimental findings. This study sheds additional light on the self-assembly of macroscopic particles in a dynamically evolving medium.

Physical Review ResearchVol. 7(1)
Wuhan University (CN)
National Science Foundation, National Natural Science Foundation of China, Wuhan University, Kavli Institute for Theoretical Physics, University of California, Santa Barbara
Openalex Percentile: Top 96%
Pickering emulsions and particle stabilization
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Self-assembling clusters of particles on a shrinking liquid surface — Duanduan Wan, Mark J. Bowick, et al. · Physical Review Research (2025) | TGRS Research Map | TGRS