Resistively detected electron spin resonance and <i>g-</i>factor in few-layer exfoliated MoS<sub>2</sub> devices

MoS<sub>2</sub>has recently emerged as a promising material for enabling quantum devices and spintronic applications. In this context, an improved physical understanding of the<i>g</i>-factor of MoS<sub>2</sub>depending on device geometry is of great importance. Resistively detected electron spin resonance (RD-ESR) could be employed to determine the<i>g</i>-factor in micron-scale devices. However, its application and RD-ESR studies have been limited by Schottky or high-resistance contacts to MoS<sub>2</sub>. Here, we exploit naturally<i>n</i>-doped few-layer MoS<sub>2</sub>devices with ohmic tin (Sn) contacts that allow the electrical study of spin phenomena. Resonant excitation of electron spins and resistive detection is a possible path to exploit the spin effects in MoS<sub>2</sub>devices. Using RD-ESR, we determine the<i>g</i>-factor of few-layer MoS<sub>2</sub>to be ∼1.92 and observe that the<i>g</i>-factor value is independent of the charge carrier density within the limits of our measurements.

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Journal
Journal of Physics Condensed Matter
Published
2025-03-20
DOI
https://doi.org/10.1088/1361-648x/adc35d
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Resistively detected electron spin resonance and g-factor in few-layer exfoliated MoS2 devices

Kai Roßnagel, L. Tiemann, Chithra H. Sharma, Jens Martin et al.
Journal of Physics Condensed Matter
2D Materials and Applications
article

Resistively detected electron spin resonance and g-factor in few-layer exfoliated MoS2 devices

Kai Roßnagel, L. Tiemann, Chithra H. Sharma, Jens Martin, Robert H. Blick, Appanna Parvangada
article en

Abstract

MoS<sub>2</sub>has recently emerged as a promising material for enabling quantum devices and spintronic applications. In this context, an improved physical understanding of the<i>g</i>-factor of MoS<sub>2</sub>depending on device geometry is of great importance. Resistively detected electron spin resonance (RD-ESR) could be employed to determine the<i>g</i>-factor in micron-scale devices. However, its application and RD-ESR studies have been limited by Schottky or high-resistance contacts to MoS<sub>2</sub>. Here, we exploit naturally<i>n</i>-doped few-layer MoS<sub>2</sub>devices with ohmic tin (Sn) contacts that allow the electrical study of spin phenomena. Resonant excitation of electron spins and resistive detection is a possible path to exploit the spin effects in MoS<sub>2</sub>devices. Using RD-ESR, we determine the<i>g</i>-factor of few-layer MoS<sub>2</sub>to be ∼1.92 and observe that the<i>g</i>-factor value is independent of the charge carrier density within the limits of our measurements.

Journal of Physics Condensed MatterVol. 37(18)
University of Wisconsin–Madison (US), Universität Hamburg (DE), Deutsches Elektronen-Synchrotron DESY (DE), Christian-Albrechts-Universität zu Kiel (DE), Leibniz Institute for Science and Mathematics Education (DE), Leibniz Institute for Crystal Growth (DE), Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE), Max Planck Institute for the Structure and Dynamics of Matter (DE)
Deutsche Forschungsgemeinschaft
Openalex Percentile: Top 96%
2D Materials and Applications
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Resistively detected electron spin resonance and <i>g-</i>factor in few-layer exfoliated MoS<sub>2</sub> devices — Kai Roßnagel, L. Tiemann, et al. · Journal of Physics Condensed Matter (2025) | TGRS Research Map | TGRS