Resistively detected electron spin resonance and <i>g-</i>factor in few-layer exfoliated MoS<sub>2</sub> devices
MoS<sub>2</sub>has recently emerged as a promising material for enabling quantum devices and spintronic applications. In this context, an improved physical understanding of the<i>g</i>-factor of MoS<sub>2</sub>depending on device geometry is of great importance. Resistively detected electron spin resonance (RD-ESR) could be employed to determine the<i>g</i>-factor in micron-scale devices. However, its application and RD-ESR studies have been limited by Schottky or high-resistance contacts to MoS<sub>2</sub>. Here, we exploit naturally<i>n</i>-doped few-layer MoS<sub>2</sub>devices with ohmic tin (Sn) contacts that allow the electrical study of spin phenomena. Resonant excitation of electron spins and resistive detection is a possible path to exploit the spin effects in MoS<sub>2</sub>devices. Using RD-ESR, we determine the<i>g</i>-factor of few-layer MoS<sub>2</sub>to be ∼1.92 and observe that the<i>g</i>-factor value is independent of the charge carrier density within the limits of our measurements.
Authors
- Kai Roßnagel (ORCID: https://orcid.org/0000-0001-5107-0090)
- L. Tiemann (ORCID: https://orcid.org/0000-0002-8588-8533)
- Chithra H. Sharma (ORCID: https://orcid.org/0000-0001-8442-5417)
- Jens Martin (ORCID: https://orcid.org/0000-0001-9548-2839)
- Robert H. Blick (ORCID: https://orcid.org/0000-0002-3602-7702)
- Appanna Parvangada
Institutions
- University of Wisconsin–Madison (US)
- Universität Hamburg (DE)
- Deutsches Elektronen-Synchrotron DESY (DE)
- Christian-Albrechts-Universität zu Kiel (DE)
- Leibniz Institute for Science and Mathematics Education (DE)
- Leibniz Institute for Crystal Growth (DE)
- Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE)
- Max Planck Institute for the Structure and Dynamics of Matter (DE)
Publication Details
- Journal
- Journal of Physics Condensed Matter
- Published
- 2025-03-20
- DOI
- https://doi.org/10.1088/1361-648x/adc35d
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Deutsche Forschungsgemeinschaft