Disorder- and Interaction-Driven Quantum Criticality in WSe<sub>2</sub>

Quantum fluctuations resulting from strong Coulomb interactions or strong disorders lead to quantum phase transitions (QPTs) in 2D materials. However, understanding of disorder- and interaction-driven QPTs remains a fundamental challenge in 2D materials owing to the presence of strong disorder and strong Coulomb interactions. Here, we study the systematic interplay of strong disorder and strong Coulomb interactions by controlling the thickness of WSe<sub>2</sub> to elucidate the disorder- and interaction-driven metal-insulator QPTs. An observation of metal-insulator transitions (MITs) with a conductivity of ∼<i>e</i><sup>2</sup>/<i>h</i> in thin-WSe<sub>2</sub> agrees with the Mott-Ioffe-Regel limit, excluding bad-metal behavior; conversely, MITs with a conductivity of <<i>e</i><sup>2</sup>/<i>h</i> demonstrate the bad-metal behavior in thick-WSe<sub>2</sub>. We observe the distinct temperature dependences of resistivity, which unveil anomalous metallic transport in WSe<sub>2</sub>. Furthermore, the emergence of the metallic glass phase (MGP) in thin-WSe<sub>2</sub> underscores the significant role of strong disorder and strong Coulomb interactions. Contrarily, the absence of the MGP in thick-WSe<sub>2</sub> suggests that the Coulomb interactions dominate over the disorder. Finally, the successful scaling collapse of conductivity reveals the disorder-dominated quantum criticality in thin-WSe<sub>2</sub> and interaction-driven Mott quantum criticality in thick-WSe<sub>2</sub>. This study provides compelling evidence that thickness-dependent WSe<sub>2</sub> could be an exciting testbed to understand anomalous metallic transport and metal-insulator QPTs in 2D materials.

Authors

Institutions

Publication Details

Journal
ACS Nano
Published
2025-03-20
DOI
https://doi.org/10.1021/acsnano.4c12942
Primary Topic
Organic and Molecular Conductors Research
Type
article
Field-Weighted Citation Impact
0.00

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Disorder- and Interaction-Driven Quantum Criticality in WSe2

Fedor Nigmatulin, Hoseong Shin, Zhipei Sun, Fida Ali et al.
ACS Nano
Organic and Molecular Conductors Research
article

Disorder- and Interaction-Driven Quantum Criticality in WSe2

Fedor Nigmatulin, Hoseong Shin, Zhipei Sun, Fida Ali, Hyokwang Park, Boseok Kang, Faisal Ahmed, Kwangro Lee, Yuqing Huang, Won Jong Yoo, Zhenping Wang, Nasir Ali, S. E. Waheed, Hyungyu Choi
article en

Abstract

Quantum fluctuations resulting from strong Coulomb interactions or strong disorders lead to quantum phase transitions (QPTs) in 2D materials. However, understanding of disorder- and interaction-driven QPTs remains a fundamental challenge in 2D materials owing to the presence of strong disorder and strong Coulomb interactions. Here, we study the systematic interplay of strong disorder and strong Coulomb interactions by controlling the thickness of WSe<sub>2</sub> to elucidate the disorder- and interaction-driven metal-insulator QPTs. An observation of metal-insulator transitions (MITs) with a conductivity of ∼<i>e</i><sup>2</sup>/<i>h</i> in thin-WSe<sub>2</sub> agrees with the Mott-Ioffe-Regel limit, excluding bad-metal behavior; conversely, MITs with a conductivity of <<i>e</i><sup>2</sup>/<i>h</i> demonstrate the bad-metal behavior in thick-WSe<sub>2</sub>. We observe the distinct temperature dependences of resistivity, which unveil anomalous metallic transport in WSe<sub>2</sub>. Furthermore, the emergence of the metallic glass phase (MGP) in thin-WSe<sub>2</sub> underscores the significant role of strong disorder and strong Coulomb interactions. Contrarily, the absence of the MGP in thick-WSe<sub>2</sub> suggests that the Coulomb interactions dominate over the disorder. Finally, the successful scaling collapse of conductivity reveals the disorder-dominated quantum criticality in thin-WSe<sub>2</sub> and interaction-driven Mott quantum criticality in thick-WSe<sub>2</sub>. This study provides compelling evidence that thickness-dependent WSe<sub>2</sub> could be an exciting testbed to understand anomalous metallic transport and metal-insulator QPTs in 2D materials.

ACS NanoVol. 19(12)
Yale University (US), Division of Materials Science and Engineering (AU), Sungkyunkwan University (KR), Aalto University (FI)
Academy of Finland, Ministry of Trade, Industry and Energy, National Research Foundation of Korea, Jane ja Aatos Erkon Säätiö, Teknologiateollisuuden 100-Vuotisjuhlasäätiö, H2020 European Research Council, H2020 Marie Skłodowska-Curie Actions
Openalex Percentile: Top 97%
Organic and Molecular Conductors Research
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.