Disorder- and Interaction-Driven Quantum Criticality in WSe<sub>2</sub>
Quantum fluctuations resulting from strong Coulomb interactions or strong disorders lead to quantum phase transitions (QPTs) in 2D materials. However, understanding of disorder- and interaction-driven QPTs remains a fundamental challenge in 2D materials owing to the presence of strong disorder and strong Coulomb interactions. Here, we study the systematic interplay of strong disorder and strong Coulomb interactions by controlling the thickness of WSe<sub>2</sub> to elucidate the disorder- and interaction-driven metal-insulator QPTs. An observation of metal-insulator transitions (MITs) with a conductivity of ∼<i>e</i><sup>2</sup>/<i>h</i> in thin-WSe<sub>2</sub> agrees with the Mott-Ioffe-Regel limit, excluding bad-metal behavior; conversely, MITs with a conductivity of <<i>e</i><sup>2</sup>/<i>h</i> demonstrate the bad-metal behavior in thick-WSe<sub>2</sub>. We observe the distinct temperature dependences of resistivity, which unveil anomalous metallic transport in WSe<sub>2</sub>. Furthermore, the emergence of the metallic glass phase (MGP) in thin-WSe<sub>2</sub> underscores the significant role of strong disorder and strong Coulomb interactions. Contrarily, the absence of the MGP in thick-WSe<sub>2</sub> suggests that the Coulomb interactions dominate over the disorder. Finally, the successful scaling collapse of conductivity reveals the disorder-dominated quantum criticality in thin-WSe<sub>2</sub> and interaction-driven Mott quantum criticality in thick-WSe<sub>2</sub>. This study provides compelling evidence that thickness-dependent WSe<sub>2</sub> could be an exciting testbed to understand anomalous metallic transport and metal-insulator QPTs in 2D materials.
Authors
- Fedor Nigmatulin (ORCID: https://orcid.org/0000-0001-9828-7086)
- Hoseong Shin
- Zhipei Sun (ORCID: https://orcid.org/0000-0002-9771-5293)
- Fida Ali (ORCID: https://orcid.org/0000-0002-0368-8213)
- Hyokwang Park
- Boseok Kang (ORCID: https://orcid.org/0000-0003-4295-3881)
- Faisal Ahmed (ORCID: https://orcid.org/0000-0002-7483-0264)
- Kwangro Lee
- Yuqing Huang (ORCID: https://orcid.org/0000-0003-4583-6365)
- Won Jong Yoo (ORCID: https://orcid.org/0000-0002-3767-7969)
- Zhenping Wang (ORCID: https://orcid.org/0000-0001-8429-7160)
- Nasir Ali (ORCID: https://orcid.org/0000-0002-6934-2186)
- S. E. Waheed
- Hyungyu Choi
Institutions
- Yale University (US)
- Division of Materials Science and Engineering (AU)
- Sungkyunkwan University (KR)
- Aalto University (FI)
Publication Details
- Journal
- ACS Nano
- Published
- 2025-03-20
- DOI
- https://doi.org/10.1021/acsnano.4c12942
- Primary Topic
- Organic and Molecular Conductors Research
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Academy of Finland
- Ministry of Trade, Industry and Energy
- National Research Foundation of Korea
- Jane ja Aatos Erkon Säätiö
- Teknologiateollisuuden 100-Vuotisjuhlasäätiö
- H2020 European Research Council
- H2020 Marie Skłodowska-Curie Actions