Disentanglement of overlapping spectrograms in attosecond time-resolved photoelectron spectroscopy of solids

Attosecond time-resolved photoelectron spectroscopy reveals photoemission dynamics, for example, via reconstruction of attosecond beating by interference of two-photon transitions (RABBITT). However, the multitude of photoemission peaks in a RABBITT spectrogram often limits the applicability of the method to well-separated photoemission channels. Here, we derive relations between RABBITT oscillations of sidebands and principal bands within strong field approximation. This allows extracting timing information on the photoemission dynamics for rather convoluted RABBITT spectra, for which the common analysis would fail. This improvement is demonstrated for simulated overlapping RABBITT spectrograms based on a solid-state photoemission model showing the robust reconstruction of the individual photoemission delays.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-03-20
DOI
https://doi.org/10.1103/physrevb.111.125146
Citations
1
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
1.25

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article

Disentanglement of overlapping spectrograms in attosecond time-resolved photoelectron spectroscopy of solids

Andreas Gebauer, Walter Pfeiffer, Tillmann Schabbehard, Luis Maschmann
1 citations
Physical review. B./Physical review. B
Laser-Matter Interactions and Applications
1.25
article

Disentanglement of overlapping spectrograms in attosecond time-resolved photoelectron spectroscopy of solids

Andreas Gebauer, Walter Pfeiffer, Tillmann Schabbehard, Luis Maschmann
article en
1 citations

Abstract

Attosecond time-resolved photoelectron spectroscopy reveals photoemission dynamics, for example, via reconstruction of attosecond beating by interference of two-photon transitions (RABBITT). However, the multitude of photoemission peaks in a RABBITT spectrogram often limits the applicability of the method to well-separated photoemission channels. Here, we derive relations between RABBITT oscillations of sidebands and principal bands within strong field approximation. This allows extracting timing information on the photoemission dynamics for rather convoluted RABBITT spectra, for which the common analysis would fail. This improvement is demonstrated for simulated overlapping RABBITT spectrograms based on a solid-state photoemission model showing the robust reconstruction of the individual photoemission delays.

Physical review. B./Physical review. BVol. 111(12)
Bielefeld University (DE)
Deutsche Forschungsgemeinschaft, Bundesministerium für Bildung und Forschung
Openalex Percentile: Top 23%
Laser-Matter Interactions and Applications
1.25
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