Excited-State Palladium-Catalyzed Radical Allylic Alkylation: Rapid Access to C2-Allyl Carbohydrates
Glycomimetics has emerged as a promising strategy to mimic the biological activities of carbohydrates while enhancing drug-like properties. Yet, their efficient synthesis and modifications remain a major challenge. Herein, we report an excited-state Pd-catalyzed, rapid synthesis of C2-allylated carbohydrates, useful synthons for preparing glycomimetics, from readily available α-bromosugars. The transformation features a high level of atom economy, broad functional group tolerance, and suitability for late-stage modification of complex molecules. Preliminary experimental and computational studies suggest a radical mechanism involving excited Pd species, 1,2-radical migration (RaM), and kinetic-controlled β-H elimination processes. We anticipate that our findings will broaden the reaction profile of excited-state Pd catalysis and enable rapid access to valuable glycomimetics.
Authors
- Peng Liu (ORCID: https://orcid.org/0000-0002-8188-632X)
- Wang Yao (ORCID: https://orcid.org/0000-0001-8708-2851)
- Jaclyn N. Mauro (ORCID: https://orcid.org/0000-0002-2018-8325)
- Ming‐Yu Ngai (ORCID: https://orcid.org/0000-0002-3055-6662)
- Yue Fu (ORCID: https://orcid.org/0000-0003-3085-7817)
- Hang Chen (ORCID: https://orcid.org/0000-0002-6699-3047)
Institutions
- State University of New York (US)
- University of Pittsburgh (US)
- Purdue University West Lafayette (US)
- Tarpo (Czechia) (CZ)
- Stony Brook University (US)
Publication Details
- Journal
- ACS Catalysis
- Published
- 2025-03-19
- DOI
- https://doi.org/10.1021/acscatal.5c00555
- Citations
- 12
- Primary Topic
- Radical Photochemical Reactions
- Type
- article
- Field-Weighted Citation Impact
- 11.23
Funders
- National Institute of General Medical Sciences
- Office of Advanced Cyberinfrastructure