Rippled metamaterials with scale-dependent tailorable elasticity

Thermally induced ripples are intrinsic features of nanometer-thick films, atomically thin materials, and cell membranes, significantly affecting their elastic properties. Despite decades of theoretical studies on the mechanics of suspended thermalized sheets, controversy still exists over the impact of these ripples, with conflicting predictions about whether elasticity is scale-dependent or scale-independent. Experimental progress has been hindered so far by the inability to have a platform capable of fully isolating and characterizing the effects of ripples. This knowledge gap limits the fundamental understanding of thin materials and their practical applications. Here, we show that thermal-like static ripples shape thin films into a class of metamaterials with scale-dependent, customizable elasticity. Utilizing a scalable semiconductor manufacturing process, we engineered nanometer-thick films with precisely controlled frozen random ripples, resembling snapshots of thermally fluctuating membranes. Resonant frequency measurements of rippled cantilevers reveal that random ripples effectively renormalize and enhance the average bending rigidity and sample-to-sample variations in a scale-dependent manner, consistent with recent theoretical estimations. The predictive power of the theoretical model, combined with the scalability of the fabrication process, was further exploited to create kirigami architectures with tailored bending rigidity and mechanical metamaterials with delayed buckling instability.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2025-03-19
DOI
https://doi.org/10.1073/pnas.2425200122
Citations
1
Primary Topic
Advanced Materials and Mechanics
Type
article
Field-Weighted Citation Impact
0.71

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article

Rippled metamaterials with scale-dependent tailorable elasticity

N. Moldovan, Daniel López, Jianguo Wen, Liliana Stan et al.
1 citations
Proceedings of the National Academy of Sciences
Advanced Materials and Mechanics
0.71
article

Rippled metamaterials with scale-dependent tailorable elasticity

N. Moldovan, Daniel López, Jianguo Wen, Liliana Stan, Andrej Košmrlj, Dafei Jin, David A. Czaplewski, Weiwei Huang, Jian Zhou, David Nelson
article en
1 citations

Abstract

Thermally induced ripples are intrinsic features of nanometer-thick films, atomically thin materials, and cell membranes, significantly affecting their elastic properties. Despite decades of theoretical studies on the mechanics of suspended thermalized sheets, controversy still exists over the impact of these ripples, with conflicting predictions about whether elasticity is scale-dependent or scale-independent. Experimental progress has been hindered so far by the inability to have a platform capable of fully isolating and characterizing the effects of ripples. This knowledge gap limits the fundamental understanding of thin materials and their practical applications. Here, we show that thermal-like static ripples shape thin films into a class of metamaterials with scale-dependent, customizable elasticity. Utilizing a scalable semiconductor manufacturing process, we engineered nanometer-thick films with precisely controlled frozen random ripples, resembling snapshots of thermally fluctuating membranes. Resonant frequency measurements of rippled cantilevers reveal that random ripples effectively renormalize and enhance the average bending rigidity and sample-to-sample variations in a scale-dependent manner, consistent with recent theoretical estimations. The predictive power of the theoretical model, combined with the scalability of the fabrication process, was further exploited to create kirigami architectures with tailored bending rigidity and mechanical metamaterials with delayed buckling instability.

Proceedings of the National Academy of SciencesVol. 122(12)
University of Notre Dame (US), Binghamton University (US), Argonne National Laboratory (US), Pennsylvania State University (US), Harvard University (US), Princeton University (US), Harvard University Press (US), Center for Nanoscale Materials
National Science Foundation, U.S. Department of Energy
Openalex Percentile: Top 35%
Advanced Materials and Mechanics
0.71
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