Overcoming temperature limitations in laser cooling using dressed states and diamond vacancies

The established approach to laser cooling of solids relies on anti-Stokes fluorescence, for example from rare earth impurities in glass. Although successful, there is a minimum temperature to which such a process can cool set by the electronic level spacing in the impurity. We propose an alternative method which does not suffer from this limitation. Our approach relies on the formation of dressed states under strong laser driving, which generates a spectrum in which the gaps can be tuned to optimize the heat absorption. This allows for a cooling cycle which operates at any temperature with a power comparable to the maximum dictated by thermodynamic principles. While this cooling cycle will compete with heating due to non-radiative decay and other mechanisms, it could in principle allow laser cooling to temperatures which are unachievable with anti-Stokes fluorescence.

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Publication Details

Published
2025-03-19
DOI
https://doi.org/10.1117/12.3041722
Primary Topic
Optical properties and cooling technologies in crystalline materials
Type
article
Field-Weighted Citation Impact
0.00

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article

Overcoming temperature limitations in laser cooling using dressed states and diamond vacancies

Conor N. Murphy, Luísa Toledo Tude, P. R. Eastham
Optical properties and cooling technologies in crystalline materials
article

Overcoming temperature limitations in laser cooling using dressed states and diamond vacancies

Conor N. Murphy, Luísa Toledo Tude, P. R. Eastham
article en

Abstract

The established approach to laser cooling of solids relies on anti-Stokes fluorescence, for example from rare earth impurities in glass. Although successful, there is a minimum temperature to which such a process can cool set by the electronic level spacing in the impurity. We propose an alternative method which does not suffer from this limitation. Our approach relies on the formation of dressed states under strong laser driving, which generates a spectrum in which the gaps can be tuned to optimize the heat absorption. This allows for a cooling cycle which operates at any temperature with a power comparable to the maximum dictated by thermodynamic principles. While this cooling cycle will compete with heating due to non-radiative decay and other mechanisms, it could in principle allow laser cooling to temperatures which are unachievable with anti-Stokes fluorescence.

Trinity College Dublin (IE)
Science Foundation Ireland, Irish Research Council
Openalex Percentile: Top 96%
Optical properties and cooling technologies in crystalline materials
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Overcoming temperature limitations in laser cooling using dressed states and diamond vacancies — Conor N. Murphy, Luísa Toledo Tude, et al. · (2025) | TGRS Research Map | TGRS