Modification of the saddle-point equation for strong-field ionization from atomic <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>p</mml:mi></mml:math> orbitals

The saddle-point approximation (SPA) within the framework of strong-field approximation is extensively applied in strong-field physics because it offers clear physical insight into intense light-matter interactions. In this study, we introduce an $m$-resolved saddle-point approximation ($m$-SPA), where $m$ is the magnetic quantum number, to analyze the ionization dynamics of atoms initially in $p$ orbitals subjected to an intense laser field. Our results reveal that $m$ influences not only the prefactor of the ionization rate but also the saddle-point equation itself, an effect overlooked in prior studies. The accuracy of the $m$-SPA method is validated through comparisons with the backpropagation method and the strong-field approximation, showing its superiority over the conventional SPA approach. By employing the $m$-SPA approach, we are able to extract more accurate distributions of the initial tunneling exit energy and position, thereby allowing for a more precise determination of the asymptotic photoelectron characteristics. Additionally, we extend the conservation law for angular momentum and energy of photoelectrons from $s$ orbitals to $p$ orbitals and from circularly polarized to elliptically polarized laser fields, both at the tunnel exit and in the asymptotic region. This work facilitates future research on strong-field ionization from arbitrary atomic orbitals.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-03-18
DOI
https://doi.org/10.1103/physreva.111.033113
Citations
3
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
3.74

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article

Modification of the saddle-point equation for strong-field ionization from atomic <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>p</mml:mi></mml:math> orbitals

Hongcheng Ni, Kunlong Liu, Xiaodan Mao, Jian Wu
3 citations
Physical review. A/Physical review, A
Laser-Matter Interactions and Applications
3.74
article

Modification of the saddle-point equation for strong-field ionization from atomic <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>p</mml:mi></mml:math> orbitals

Hongcheng Ni, Kunlong Liu, Xiaodan Mao, Jian Wu
article en
3 citations

Abstract

The saddle-point approximation (SPA) within the framework of strong-field approximation is extensively applied in strong-field physics because it offers clear physical insight into intense light-matter interactions. In this study, we introduce an $m$-resolved saddle-point approximation ($m$-SPA), where $m$ is the magnetic quantum number, to analyze the ionization dynamics of atoms initially in $p$ orbitals subjected to an intense laser field. Our results reveal that $m$ influences not only the prefactor of the ionization rate but also the saddle-point equation itself, an effect overlooked in prior studies. The accuracy of the $m$-SPA method is validated through comparisons with the backpropagation method and the strong-field approximation, showing its superiority over the conventional SPA approach. By employing the $m$-SPA approach, we are able to extract more accurate distributions of the initial tunneling exit energy and position, thereby allowing for a more precise determination of the asymptotic photoelectron characteristics. Additionally, we extend the conservation law for angular momentum and energy of photoelectrons from $s$ orbitals to $p$ orbitals and from circularly polarized to elliptically polarized laser fields, both at the tunnel exit and in the asymptotic region. This work facilitates future research on strong-field ionization from arbitrary atomic orbitals.

Physical review. A/Physical review, AVol. 111(3)
Shanxi University of Traditional Chinese Medicine (CN), Great Bay University, East China Normal University (CN)
National Natural Science Foundation of China, Science and Technology Commission of Shanghai Municipality
Openalex Percentile: Top 8%
Laser-Matter Interactions and Applications
3.74
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