Long-Range Coherent Emission of Propagating Exciton–Polaritons from a Mach–Zehnder Interferometer

Long-range coherence of the part-matter, part-light exciton–polariton has potential applications in all-optical logic that combine the large nonlinearity of the matter component with the delocalization by the light component. A polariton condensate has been shown to have long-range coherence, although the formation of a condensate requires complex device fabrication and well-defined operation conditions. In this work, we demonstrate a Mach–Zehnder interferometer that exhibits room-temperature, long-range coherent propagation of Bloch surface wave polaritons (BSWPs) that does not depend on the formation of a condensate. Due to strong coupling of the organic exciton and the delocalized BSW supported by a distributed Bragg reflector (DBR), the hybrid light–matter states sustain coherence over distances of ∼50 μm, giving rise to wavelength-dependent interference patterns within the devices. Our results show that the BSWP represents a promising platform for room-temperature coherent polaritonic devices, thus enabling integrated photonic circuits that operate under ambient conditions.

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Publication Details

Journal
ACS Photonics
Published
2025-03-18
DOI
https://doi.org/10.1021/acsphotonics.4c02442
Citations
1
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
1.25

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article

Long-Range Coherent Emission of Propagating Exciton–Polaritons from a Mach–Zehnder Interferometer

Jeffrey C. Horowitz, Stephen R. Forrest, Sritoma Paul, Bin Liu
1 citations
ACS Photonics
Strong Light-Matter Interactions
1.25
article

Long-Range Coherent Emission of Propagating Exciton–Polaritons from a Mach–Zehnder Interferometer

Jeffrey C. Horowitz, Stephen R. Forrest, Sritoma Paul, Bin Liu
article en
1 citations

Abstract

Long-range coherence of the part-matter, part-light exciton–polariton has potential applications in all-optical logic that combine the large nonlinearity of the matter component with the delocalization by the light component. A polariton condensate has been shown to have long-range coherence, although the formation of a condensate requires complex device fabrication and well-defined operation conditions. In this work, we demonstrate a Mach–Zehnder interferometer that exhibits room-temperature, long-range coherent propagation of Bloch surface wave polaritons (BSWPs) that does not depend on the formation of a condensate. Due to strong coupling of the organic exciton and the delocalized BSW supported by a distributed Bragg reflector (DBR), the hybrid light–matter states sustain coherence over distances of ∼50 μm, giving rise to wavelength-dependent interference patterns within the devices. Our results show that the BSWP represents a promising platform for room-temperature coherent polaritonic devices, thus enabling integrated photonic circuits that operate under ambient conditions.

ACS PhotonicsVol. 12(4)
University of Michigan (US)
Universal Display Corporation
Openalex Percentile: Top 23%
Strong Light-Matter Interactions
1.25
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Long-Range Coherent Emission of Propagating Exciton–Polaritons from a Mach–Zehnder Interferometer — Jeffrey C. Horowitz, Stephen R. Forrest, et al. · ACS Photonics (2025) | TGRS Research Map | TGRS