Reaction-limited evaporation for the color-gradient lattice Boltzmann model

We propose a reaction-limited evaporation model within the color-gradient lattice Boltzmann (LB) multicomponent framework to address the lack of intrinsic evaporation mechanisms. Unlike diffusion-driven approaches, our method directly enforces mass removal at the fluid interface in a reaction-limited manner while maintaining numerical stability. Using the inherent color-gradient magnitude and a single adjustable parameter, evaporation sites are chosen in a computationally efficient way with seamless mass exchange between the components, with no change to the core algorithm. Extensive validation across diverse interface geometries and evaporation flux magnitudes demonstrates high accuracy, with errors below 5% for unit density ratios. For density contrasts, the method remains robust in the limit of smaller evaporation flux magnitudes and density ratios. Our approach extends the applicability of the color-gradient LB model to scenarios involving reaction-limited evaporation, such as droplet evaporation on heated substrates, vacuum evaporation of molten metals, and drying processes in porous media.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2025-03-18
DOI
https://doi.org/10.1063/5.0253799
Citations
2
Primary Topic
Nanomaterials and Printing Technologies
Type
article
Field-Weighted Citation Impact
1.46

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article

Reaction-limited evaporation for the color-gradient lattice Boltzmann model

Othmane Aouane, Jens Harting, Gaurav Nath
2 citations
The Journal of Chemical Physics
Nanomaterials and Printing Technologies
1.46
article

Reaction-limited evaporation for the color-gradient lattice Boltzmann model

Othmane Aouane, Jens Harting, Gaurav Nath
article en
2 citations

Abstract

We propose a reaction-limited evaporation model within the color-gradient lattice Boltzmann (LB) multicomponent framework to address the lack of intrinsic evaporation mechanisms. Unlike diffusion-driven approaches, our method directly enforces mass removal at the fluid interface in a reaction-limited manner while maintaining numerical stability. Using the inherent color-gradient magnitude and a single adjustable parameter, evaporation sites are chosen in a computationally efficient way with seamless mass exchange between the components, with no change to the core algorithm. Extensive validation across diverse interface geometries and evaporation flux magnitudes demonstrates high accuracy, with errors below 5% for unit density ratios. For density contrasts, the method remains robust in the limit of smaller evaporation flux magnitudes and density ratios. Our approach extends the applicability of the color-gradient LB model to scenarios involving reaction-limited evaporation, such as droplet evaporation on heated substrates, vacuum evaporation of molten metals, and drying processes in porous media.

The Journal of Chemical PhysicsVol. 162(11)
Friedrich-Alexander-Universität Erlangen-Nürnberg (DE), Helmholtz Institute Erlangen-Nürnberg (DE)
Deutsche Forschungsgemeinschaft
Life below water
Openalex Percentile: Top 19%
Nanomaterials and Printing Technologies
1.46
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Reaction-limited evaporation for the color-gradient lattice Boltzmann model — Othmane Aouane, Jens Harting, et al. · The Journal of Chemical Physics (2025) | TGRS Research Map | TGRS