Using Light to Polarize and Detect Electron Spins in Silicon

Despite decades of research, demonstration of all-optical detection and control of free electron spins in silicon remains elusive. Here, we directly probe the electron spin properties in bulk silicon by measuring the polarization of luminescence following circularly polarized light excitation. The all-optical experiments performed for both direct and indirect gap excitation allow not only an experimental determination of the optical selection rules in silicon for the different phonon-assisted transitions but they also lead to the measurement of the spin relaxation of electrons in conditions that are not accessible using transport techniques. We also measure the spin properties of free excitons in bulk silicon, a very little explored field.

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Publication Details

Journal
Physical Review Letters
Published
2025-03-14
DOI
https://doi.org/10.1103/physrevlett.134.106902
Citations
1
Primary Topic
Quantum and electron transport phenomena
Type
article
Field-Weighted Citation Impact
1.25

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Using Light to Polarize and Detect Electron Spins in Silicon

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Quantum and electron transport phenomena
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Using Light to Polarize and Detect Electron Spins in Silicon

Fabian Cadiz, X. Marie, A. Balocchi, T. Amand, P. Renucci, Delphine Lagarde, Laurent Lombez, C. Robert
article en
1 citations

Abstract

Despite decades of research, demonstration of all-optical detection and control of free electron spins in silicon remains elusive. Here, we directly probe the electron spin properties in bulk silicon by measuring the polarization of luminescence following circularly polarized light excitation. The all-optical experiments performed for both direct and indirect gap excitation allow not only an experimental determination of the optical selection rules in silicon for the different phonon-assisted transitions but they also lead to the measurement of the spin relaxation of electrons in conditions that are not accessible using transport techniques. We also measure the spin properties of free excitons in bulk silicon, a very little explored field.

Physical Review LettersVol. 134(10)
École Polytechnique (FR), Université Fédérale de Toulouse Midi-Pyrénées (FR), Institut Universitaire de France (FR), Laboratoire de Physique Théorique de la Matière Condensée (FR), Institut Polytechnique de Paris (FR), Laboratoire de Physique et Chimie des Nano-Objets (FR), Laboratoire de physique de la matière condensée (FR)
Agence Nationale de la Recherche
Affordable and clean energy
Openalex Percentile: Top 23%
Quantum and electron transport phenomena
1.25
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