Reconfigurable Terahertz Metamaterials Based on the Refractive Index Change of Epitaxial Vanadium Dioxide Films Across the Metal–Insulator Transition

The intrinsic metal-insulator transition (MIT) of VO<sub>2</sub> films near room temperature presents significant potential for reconfigurable metamaterials in the terahertz (THz) frequency range. While previous designs primarily focused on changes in electrical conductivity across the MIT, the accompanying dielectric changes due to the mesoscopic carrier confinement effect have been largely unexplored. In this study, we integrate asymmetric split-ring resonators on 35 nm epitaxial VO<sub>2</sub> film and identify a "dielectric window" at the early stages of the MIT. This is characterized by a redshift in the resonant frequency without a significant degradation in the resonant quality. This phenomenon is attributed to an inhomogeneous phase transition in the VO<sub>2</sub> film, which induces a purely dielectric change at the onset of the MIT, while the electrical conductivity transition occurs later, slightly above the percolation threshold. Our findings provide deeper insights into the THz properties of VO<sub>2</sub> films and pave the way for dielectric-based, VO<sub>2</sub> hybrid reconfigurable metamaterials.

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Publication Details

Journal
Nanomaterials
Published
2025-03-13
DOI
https://doi.org/10.3390/nano15060439
Citations
1
Primary Topic
Transition Metal Oxide Nanomaterials
Type
article
Field-Weighted Citation Impact
0.61
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article

Reconfigurable Terahertz Metamaterials Based on the Refractive Index Change of Epitaxial Vanadium Dioxide Films Across the Metal–Insulator Transition

Weizheng Liang, Chang Lu
1 citations
Nanomaterials
Transition Metal Oxide Nanomaterials
0.61
article

Reconfigurable Terahertz Metamaterials Based on the Refractive Index Change of Epitaxial Vanadium Dioxide Films Across the Metal–Insulator Transition

Weizheng Liang, Chang Lu
article en
1 citations

Abstract

The intrinsic metal-insulator transition (MIT) of VO<sub>2</sub> films near room temperature presents significant potential for reconfigurable metamaterials in the terahertz (THz) frequency range. While previous designs primarily focused on changes in electrical conductivity across the MIT, the accompanying dielectric changes due to the mesoscopic carrier confinement effect have been largely unexplored. In this study, we integrate asymmetric split-ring resonators on 35 nm epitaxial VO<sub>2</sub> film and identify a "dielectric window" at the early stages of the MIT. This is characterized by a redshift in the resonant frequency without a significant degradation in the resonant quality. This phenomenon is attributed to an inhomogeneous phase transition in the VO<sub>2</sub> film, which induces a purely dielectric change at the onset of the MIT, while the electrical conductivity transition occurs later, slightly above the percolation threshold. Our findings provide deeper insights into the THz properties of VO<sub>2</sub> films and pave the way for dielectric-based, VO<sub>2</sub> hybrid reconfigurable metamaterials.

NanomaterialsVol. 15(6)
Guangxi University (CN), Shenzhen Institute of Information Technology (CN)
Openalex Percentile: Top 39%
Transition Metal Oxide Nanomaterials
0.61
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