Enhanced magnetic ordering in the heavy lanthanide Er metal under megabar pressures

Four-point electrical resistivity measurements were carried out on erbium (Er) metal and dilute magnetic alloy containing 0.5 at.$%$ Er in superconducting Y for temperatures 3.5--295 K under pressures to 183 GPa in a diamond anvil cell. The magnetic ordering temperature ${T}_{o}$ of Er appears to rise rapidly above 80 GPa. Y(Er) alloys display giant superconducting pair breaking $\mathrm{\ensuremath{\Delta}}{T}_{c}$ per atomic percent as large as 19 K/at.$%$ Er. The present results give evidence that, for pressures above 80 GPa, the exchange coupling $J$ between Er ions and conduction electrons becomes negative, thus activating Kondo physics in this highly correlated electron system. We suggest that these anomalously high magnetic ordering temperatures are an unrecognized feature of the Kondo lattice state, providing another perspective for designing magnetic materials with high ordering temperature.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-03-07
DOI
https://doi.org/10.1103/physrevb.111.125117
Citations
1
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
1.26

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article

Enhanced magnetic ordering in the heavy lanthanide Er metal under megabar pressures

Jing Song, Baosen Min, Changqing Jin, Wei Wu et al.
1 citations
Physical review. B./Physical review. B
Rare-earth and actinide compounds
1.26
article

Enhanced magnetic ordering in the heavy lanthanide Er metal under megabar pressures

Jing Song, Baosen Min, Changqing Jin, Wei Wu, Sijia Zhang, Xiancheng Wang, Hongyu Liu, Shaomin Feng
article en
1 citations

Abstract

Four-point electrical resistivity measurements were carried out on erbium (Er) metal and dilute magnetic alloy containing 0.5 at.$%$ Er in superconducting Y for temperatures 3.5--295 K under pressures to 183 GPa in a diamond anvil cell. The magnetic ordering temperature ${T}_{o}$ of Er appears to rise rapidly above 80 GPa. Y(Er) alloys display giant superconducting pair breaking $\mathrm{\ensuremath{\Delta}}{T}_{c}$ per atomic percent as large as 19 K/at.$%$ Er. The present results give evidence that, for pressures above 80 GPa, the exchange coupling $J$ between Er ions and conduction electrons becomes negative, thus activating Kondo physics in this highly correlated electron system. We suggest that these anomalously high magnetic ordering temperatures are an unrecognized feature of the Kondo lattice state, providing another perspective for designing magnetic materials with high ordering temperature.

Physical review. B./Physical review. BVol. 111(12)
Chinese Academy of Sciences (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), University of Chinese Academy of Sciences (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 24%
Rare-earth and actinide compounds
1.26
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