In Situ TEM Study of Size-Controlled Bi Quantum Dots in an Annealed GaAsBi/AlAs Multiple Quantum Well Structure

An in situ transmission electron microscopy study of Bi quantum dot (QD) formation in an annealed GaAsBi/AlAs multiple quantum well (MQW) structure is presented in this work. The investigated structure, containing two GaAsBi QWs and embedded in an AlGaAs parabolic quantum barrier (PQB), was grown on semi-insulating GaAs (100) and was transferred onto an in situ heating holder (DENS solutions) and heated up to 650 °C. Sample evolution was continuously recorded in situ in bright-field STEM mode. The analysis revealed that QD formation occurs at lower annealing temperatures in case of <i>in situ</i> heating of lamella than in bulk. In addition, we find that the mechanism governing Bi QD formation is different in the in situ TEM experiment compared to bulk ex-situ annealing. Comparison of the <i>ex-situ</i> and <i>in situ</i> annealed structures, as well as in-depth postannealed structure TEM analysis, is presented.

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Publication Details

Journal
ACS Omega
Published
2025-03-06
DOI
https://doi.org/10.1021/acsomega.4c10631
Citations
3
Primary Topic
Semiconductor Quantum Structures and Devices
Type
article
Field-Weighted Citation Impact
3.74

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article

In Situ TEM Study of Size-Controlled Bi Quantum Dots in an Annealed GaAsBi/AlAs Multiple Quantum Well Structure

Renata Butkutė, Sandra Stanionytė, Martynas Skapas, E. Luna et al.
3 citations
ACS Omega
Semiconductor Quantum Structures and Devices
3.74
article

In Situ TEM Study of Size-Controlled Bi Quantum Dots in an Annealed GaAsBi/AlAs Multiple Quantum Well Structure

Renata Butkutė, Sandra Stanionytė, Martynas Skapas, E. Luna, Karl Graser
article en
3 citations

Abstract

An in situ transmission electron microscopy study of Bi quantum dot (QD) formation in an annealed GaAsBi/AlAs multiple quantum well (MQW) structure is presented in this work. The investigated structure, containing two GaAsBi QWs and embedded in an AlGaAs parabolic quantum barrier (PQB), was grown on semi-insulating GaAs (100) and was transferred onto an in situ heating holder (DENS solutions) and heated up to 650 °C. Sample evolution was continuously recorded in situ in bright-field STEM mode. The analysis revealed that QD formation occurs at lower annealing temperatures in case of <i>in situ</i> heating of lamella than in bulk. In addition, we find that the mechanism governing Bi QD formation is different in the in situ TEM experiment compared to bulk ex-situ annealing. Comparison of the <i>ex-situ</i> and <i>in situ</i> annealed structures, as well as in-depth postannealed structure TEM analysis, is presented.

ACS OmegaVol. 10(10)
Center for Physical Sciences and Technology (LT), Paul Drude Institute for Solid State Electronics (DE)
Lietuvos Mokslo Taryba
Openalex Percentile: Top 8%
Semiconductor Quantum Structures and Devices
3.74
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In Situ TEM Study of Size-Controlled Bi Quantum Dots in an Annealed GaAsBi/AlAs Multiple Quantum Well Structure — Renata Butkutė, Sandra Stanionytė, et al. · ACS Omega (2025) | TGRS Research Map | TGRS