High-Performance Planar Thin-Film Thermoelectric Cooler Based on Sputtered Nanocrystalline Bi<sub>2</sub>Te<sub>3</sub>/Bi<sub>0.5</sub>Sb<sub>1.5</sub>Te<sub>3</sub> Thin Films for On-Chip Cooling

The development of high-performance thin-film thermoelectric coolers (TFTECs) that are compatible with standard integrated circuit processes and can reduce power consumption is critical to achieving large-scale applications. In this work, we fabricate a planar TFTEC based on nanocrystalline p-type Bi<sub>0.5</sub>Sb<sub>1.5</sub>Te<sub>3</sub> and n-type Bi<sub>2</sub>Te<sub>3</sub> thin films using magnetron sputtering, standard lithography, and postannealing processes. The power factors of the Bi<sub>0.5</sub>Sb<sub>1.5</sub>Te<sub>3</sub> and Bi<sub>2</sub>Te<sub>3</sub> thin films reach 3.63 and 4.28 mW/mK<sup>2</sup>, respectively, and the ZT values reach 0.82 and 0.93, which are comparable to those of bulk TE materials. The radial configuration of the device allows the cold-side thermal resistance to be increased and the hot-side thermal resistance to be decreased, thereby facilitating a substantial cooling temperature difference. Furthermore, the large in-plane contact area helps to reduce device resistance and power consumption. At a heating stage temperature of 360 K and a power consumption of 4.76 mW, the net cooling temperature difference of the TFTEC reaches 4 °C. The maximum temperature difference between the hot end and the cold end is 7.26 °C, while the cold end temperature remains below the ambient temperature. The high-performance planar TFTECs demonstrated in this work exhibit both a high net cooling performance and competitive fabrication cost, rendering them ideal for on-chip hotspot cooling.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2025-03-05
DOI
https://doi.org/10.1021/acsami.4c19653
Citations
10
Primary Topic
Advanced Thermoelectric Materials and Devices
Type
article
Field-Weighted Citation Impact
5.18

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article

High-Performance Planar Thin-Film Thermoelectric Cooler Based on Sputtered Nanocrystalline Bi2Te3/Bi0.5Sb1.5Te3 Thin Films for On-Chip Cooling

Linwei Cao, Lei Gao, Jun‐Tao Li, Maolin Shi et al.
10 citations
ACS Applied Materials & Interfaces
Advanced Thermoelectric Materials and Devices
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article

High-Performance Planar Thin-Film Thermoelectric Cooler Based on Sputtered Nanocrystalline Bi2Te3/Bi0.5Sb1.5Te3 Thin Films for On-Chip Cooling

Linwei Cao, Lei Gao, Jun‐Tao Li, Maolin Shi, Tingrui Gong, Wei Su, Lianghui Li, Chensheng Ma
article en
10 citations

Abstract

The development of high-performance thin-film thermoelectric coolers (TFTECs) that are compatible with standard integrated circuit processes and can reduce power consumption is critical to achieving large-scale applications. In this work, we fabricate a planar TFTEC based on nanocrystalline p-type Bi<sub>0.5</sub>Sb<sub>1.5</sub>Te<sub>3</sub> and n-type Bi<sub>2</sub>Te<sub>3</sub> thin films using magnetron sputtering, standard lithography, and postannealing processes. The power factors of the Bi<sub>0.5</sub>Sb<sub>1.5</sub>Te<sub>3</sub> and Bi<sub>2</sub>Te<sub>3</sub> thin films reach 3.63 and 4.28 mW/mK<sup>2</sup>, respectively, and the ZT values reach 0.82 and 0.93, which are comparable to those of bulk TE materials. The radial configuration of the device allows the cold-side thermal resistance to be increased and the hot-side thermal resistance to be decreased, thereby facilitating a substantial cooling temperature difference. Furthermore, the large in-plane contact area helps to reduce device resistance and power consumption. At a heating stage temperature of 360 K and a power consumption of 4.76 mW, the net cooling temperature difference of the TFTEC reaches 4 °C. The maximum temperature difference between the hot end and the cold end is 7.26 °C, while the cold end temperature remains below the ambient temperature. The high-performance planar TFTECs demonstrated in this work exhibit both a high net cooling performance and competitive fabrication cost, rendering them ideal for on-chip hotspot cooling.

ACS Applied Materials & InterfacesVol. 17(11)
China Academy of Engineering Physics (CN)
National Natural Science Foundation of China
Affordable and clean energy
Openalex Percentile: Top 4%
Advanced Thermoelectric Materials and Devices
5.18
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