Minimizing interference in low-pressure supersonic beam sources

Free-jet atomic, cluster, and molecular sources are typically used to produce beams of low-energy, neutral particles and find application in a wide array of technologies, from neutral atom microscopes to instruments for surface processing. We present a simple analytical theory that is applicable to many of these sources, when (i) the nozzle-skimmer distance is such that free molecular flow is achieved and (ii) there is negligible interference within the skimmer itself. The utility of the model is demonstrated by comparing experimental data with calculations performed using the theory. In particular, we show that skimmer interference is negligible compared to attenuation by "background" gas for room-temperature beams. Our treatment does not depend on any free parameters and obviates the complexity of previous theories. As a result, we are able to devise a number of design recommendations to minimize interference in sources operating with cryogenic-temperature beams.

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Publication Details

Journal
The Journal of Chemical Physics
Published
2025-03-04
DOI
https://doi.org/10.1063/5.0247870
Citations
1
Primary Topic
Gas Dynamics and Kinetic Theory
Type
article
Field-Weighted Citation Impact
3.73

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article

Minimizing interference in low-pressure supersonic beam sources

Jack Kelsall, J. Ellis, Aleksandar Radić, A. P. Jardine et al.
1 citations
The Journal of Chemical Physics
Gas Dynamics and Kinetic Theory
3.73
article

Minimizing interference in low-pressure supersonic beam sources

Jack Kelsall, J. Ellis, Aleksandar Radić, A. P. Jardine, David J. Ward
article en
1 citations

Abstract

Free-jet atomic, cluster, and molecular sources are typically used to produce beams of low-energy, neutral particles and find application in a wide array of technologies, from neutral atom microscopes to instruments for surface processing. We present a simple analytical theory that is applicable to many of these sources, when (i) the nozzle-skimmer distance is such that free molecular flow is achieved and (ii) there is negligible interference within the skimmer itself. The utility of the model is demonstrated by comparing experimental data with calculations performed using the theory. In particular, we show that skimmer interference is negligible compared to attenuation by "background" gas for room-temperature beams. Our treatment does not depend on any free parameters and obviates the complexity of previous theories. As a result, we are able to devise a number of design recommendations to minimize interference in sources operating with cryogenic-temperature beams.

The Journal of Chemical PhysicsVol. 162(9)
University of Cambridge (GB), Bridge University (SS)
Engineering and Physical Sciences Research Council, Innovate UK
Affordable and clean energy
Openalex Percentile: Top 12%
Gas Dynamics and Kinetic Theory
3.73
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Minimizing interference in low-pressure supersonic beam sources — Jack Kelsall, J. Ellis, et al. · The Journal of Chemical Physics (2025) | TGRS Research Map | TGRS