Minimization of temperature reached by adiabatic demagnetization refrigeration in Ce-based intermetallic Ce2(Cu1<b>−</b> <i>x</i>Ni<i>x</i>)2In

Magnetic entropy remaining near absolute zero temperature in the antiferromagnetic (AFM) critical state is expected to be usable for the cryogenic magnetic refrigeration. In this paper, we report quasi-adiabatic demagnetization refrigeration for Ce2(Cu1−xNix)2In (0≤x≤0.38) whose parent compound Ce2Cu2In orders antiferromagnetically below 6 K, by using a laboratory-made cell attachable to a commercial 4He refrigerator with a base temperature of 1.8 K. The final temperature by the quasi-adiabatic demagnetization as a function of x indicates a local minimum of 1 K at the AFM critical composition of x∼0.3. The validity of this result is confirmed by our specific-heat measurements. Our work motivates the future developments of Ce-based cryogenic magnetic refrigerants with the lower characteristic temperature in view of the low cost and easiness in synthesizing compared with Yb-based counterparts.

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Publication Details

Journal
Applied Physics Letters
Published
2025-03-01
DOI
https://doi.org/10.1063/5.0245318
Citations
3
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
3.77

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article

Minimization of temperature reached by adiabatic demagnetization refrigeration in Ce-based intermetallic Ce2(Cu1− xNix)2In

Kanta Watanabe, Yasuyuki Shimura, Kazunori Umeo, Takahiro Onimaru et al.
3 citations
Applied Physics Letters
Rare-earth and actinide compounds
3.77
article

Minimization of temperature reached by adiabatic demagnetization refrigeration in Ce-based intermetallic Ce2(Cu1− xNix)2In

Kanta Watanabe, Yasuyuki Shimura, Kazunori Umeo, Takahiro Onimaru, T. Takabatake
article en
3 citations

Abstract

Magnetic entropy remaining near absolute zero temperature in the antiferromagnetic (AFM) critical state is expected to be usable for the cryogenic magnetic refrigeration. In this paper, we report quasi-adiabatic demagnetization refrigeration for Ce2(Cu1−xNix)2In (0≤x≤0.38) whose parent compound Ce2Cu2In orders antiferromagnetically below 6 K, by using a laboratory-made cell attachable to a commercial 4He refrigerator with a base temperature of 1.8 K. The final temperature by the quasi-adiabatic demagnetization as a function of x indicates a local minimum of 1 K at the AFM critical composition of x∼0.3. The validity of this result is confirmed by our specific-heat measurements. Our work motivates the future developments of Ce-based cryogenic magnetic refrigerants with the lower characteristic temperature in view of the low cost and easiness in synthesizing compared with Yb-based counterparts.

Applied Physics LettersVol. 126(9)
Hiroshima University (JP)
Mazda Foundation, Hattori Hokokai Foundation, Japan Society for the Promotion of Science, Fusion Oriented REsearch for disruptive Science and Technology
Openalex Percentile: Top 8%
Rare-earth and actinide compounds
3.77
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Minimization of temperature reached by adiabatic demagnetization refrigeration in Ce-based intermetallic Ce2(Cu1<b>−</b> <i>x</i>Ni<i>x</i>)2In — Kanta Watanabe, Yasuyuki Shimura, et al. · Applied Physics Letters (2025) | TGRS Research Map | TGRS