Minimization of temperature reached by adiabatic demagnetization refrigeration in Ce-based intermetallic Ce2(Cu1<b>−</b> <i>x</i>Ni<i>x</i>)2In
Magnetic entropy remaining near absolute zero temperature in the antiferromagnetic (AFM) critical state is expected to be usable for the cryogenic magnetic refrigeration. In this paper, we report quasi-adiabatic demagnetization refrigeration for Ce2(Cu1−xNix)2In (0≤x≤0.38) whose parent compound Ce2Cu2In orders antiferromagnetically below 6 K, by using a laboratory-made cell attachable to a commercial 4He refrigerator with a base temperature of 1.8 K. The final temperature by the quasi-adiabatic demagnetization as a function of x indicates a local minimum of 1 K at the AFM critical composition of x∼0.3. The validity of this result is confirmed by our specific-heat measurements. Our work motivates the future developments of Ce-based cryogenic magnetic refrigerants with the lower characteristic temperature in view of the low cost and easiness in synthesizing compared with Yb-based counterparts.
Authors
- Kanta Watanabe
- Yasuyuki Shimura (ORCID: https://orcid.org/0000-0002-2598-1277)
- Kazunori Umeo (ORCID: https://orcid.org/0000-0001-9442-4143)
- Takahiro Onimaru (ORCID: https://orcid.org/0000-0001-9990-3098)
- T. Takabatake (ORCID: https://orcid.org/0000-0002-3293-8592)
Institutions
- Hiroshima University (JP)
Publication Details
- Journal
- Applied Physics Letters
- Published
- 2025-03-01
- DOI
- https://doi.org/10.1063/5.0245318
- Citations
- 3
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 3.77
Funders
- Mazda Foundation
- Hattori Hokokai Foundation
- Japan Society for the Promotion of Science
- Fusion Oriented REsearch for disruptive Science and Technology