Fate of transient order parameter domain walls in ultrafast experiments

In ultrafast experiments, an optical pump pulse often generates transient domain walls of the order parameter in materials with spontaneous symmetry breaking, due to either a finite penetration depth of light on a three-dimensional (3D) material, or a finite spot size on a two-dimensional (2D) material. We show that the domain wall decays due to unstable order parameter fluctuations. We study a generic system with U(1)-symmetric order, and those with an additional weak Z2 (U(1)-symmetry-breaking) term, representing the charge-density-wave (CDW) orders in recent experiments. During the first stage of the decay dynamics, exponentially growing thermal fluctuations convert the domain wall into an interface with randomly distributed topological defects. In the second stage, the topological defects undergo a coarsening dynamics within the interface. For a 2D interface in a 3D system, the coarsening dynamics leads to a diffusive growth of the correlation length. For a one-dimensional (1D) interface in a 2D system with the weak Z2 term, the correlation-length growth shows a crossover from diffusive to sub-diffusive behavior.

Authors

Institutions

Publication Details

Journal
npj Quantum Materials
Published
2025-02-27
DOI
https://doi.org/10.1038/s41535-025-00743-w
Citations
1
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
1.25

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Fate of transient order parameter domain walls in ultrafast experiments

Zhiyuan Sun, Lingxian Kong, Ryuichi Shindou
1 citations
npj Quantum Materials
Mechanical and Optical Resonators
1.25
article

Fate of transient order parameter domain walls in ultrafast experiments

Zhiyuan Sun, Lingxian Kong, Ryuichi Shindou
article en
1 citations

Abstract

In ultrafast experiments, an optical pump pulse often generates transient domain walls of the order parameter in materials with spontaneous symmetry breaking, due to either a finite penetration depth of light on a three-dimensional (3D) material, or a finite spot size on a two-dimensional (2D) material. We show that the domain wall decays due to unstable order parameter fluctuations. We study a generic system with U(1)-symmetric order, and those with an additional weak Z2 (U(1)-symmetry-breaking) term, representing the charge-density-wave (CDW) orders in recent experiments. During the first stage of the decay dynamics, exponentially growing thermal fluctuations convert the domain wall into an interface with randomly distributed topological defects. In the second stage, the topological defects undergo a coarsening dynamics within the interface. For a 2D interface in a 3D system, the coarsening dynamics leads to a diffusive growth of the correlation length. For a one-dimensional (1D) interface in a 2D system with the weak Z2 term, the correlation-length growth shows a crossover from diffusive to sub-diffusive behavior.

npj Quantum MaterialsVol. 10(1)
Peking University (CN), Tsinghua University (CN)
National Natural Science Foundation of China
Climate action
Openalex Percentile: Top 24%
Mechanical and Optical Resonators
1.25
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.