Hydrogel In-Tape Electronic Tongue
An electronic tongue is a sensor-based system designed to mimic human taste by detecting and analyzing the chemical properties of liquids through electrochemical methods. Here, we introduce the HITS concept, an electronic tongue system that enables rapid and sequential classification of various beverages. This system utilizes a single, cost-effective platform with interdigital electrodes made of carbon printed on recyclable poly(ethylene terephthalate) (PET), significantly reducing the need for multiple electrodes. With the use of interchangeable hydrogel tapes, the system requires a single deep (150 μL) pore per analysis, allowing for efficient sequential testing. The hydrogel seamlessly accommodates the electrode interface and operates with a semisolid electrolyte, achieving ultrafast analysis times of just 5 min. Employing AI and machine learning algorithms, HITS accurately differentiated between coffee, juice, water, white wine, and red wine with a 100% success rate. This sustainable approach combines high precision, speed, and low environmental impact, offering a versatile solution for various technological applications, including food science, quality control, and health monitoring. This e-solution not only enhances precision and speed but also aligns with growing environmental concerns, offering a low-impact and scalable platform for advanced liquid analysis.
Authors
- Clarisse Ribeiro (ORCID: https://orcid.org/0000-0002-9120-4847)
- Rita Polícia (ORCID: https://orcid.org/0000-0003-1635-0665)
- Senentxu Lanceros-Méndez (ORCID: https://orcid.org/0000-0001-6791-7620)
- Ricardo Brito‐Pereira (ORCID: https://orcid.org/0000-0002-0983-2415)
- P. Martins (ORCID: https://orcid.org/0000-0002-9833-9648)
- Frank N. Crespilho (ORCID: https://orcid.org/0000-0003-4830-652X)
Institutions
- Ikerbasque (ES)
- Basque Center for Materials, Applications and Nanostructures (ES)
- Vitenparken (NO)
- University of Minho (PT)
Publication Details
- Journal
- ACS Applied Electronic Materials
- Published
- 2025-02-26
- DOI
- https://doi.org/10.1021/acsaelm.4c02059
- Citations
- 4
- Primary Topic
- Advanced Sensor and Energy Harvesting Materials
- Type
- article
- Field-Weighted Citation Impact
- 2.70
Funders
- Ministerio de Ciencia, Innovación y Universidades
- Fundação de Amparo à Pesquisa do Estado de São Paulo
- Coordenação de Aperfeiçoamento de Pessoal de Nível Superior
- Eusko Jaurlaritza
- Ministerio de Economía y Competitividad
- Fundação para a Ciência e a Tecnologia