Anomalous temperature dependence of spin–orbit coupling in Al<sub>2</sub>O<sub>3</sub>/SrTiO<sub>3</sub> and Al<sub>2</sub>O<sub>3</sub>/KTaO<sub>3</sub> heterostructures

Perovskite oxide-based heterostructures exhibit a range of exotic physical properties such as two-dimensional superconductivity, interface magnetism, tunable Kondo effect, and tunable spin-orbit coupling. Here, the magnetotransport properties of Al<sub>2</sub>O<sub>3</sub>/SrTiO<sub>3</sub>and Al<sub>2</sub>O<sub>3</sub>/KTaO<sub>3</sub>heterostructures are studied. Both Kondo effect and spin-orbit coupling-induced weak antilocalization (WAL) effect are observed at low temperatures. By analyzing the WAL curves, the spin relaxation time is extracted. Surprisingly, the extracted spin relaxation time unexpectedly decreases on increasing temperature in all samples. This indicates that the strength of the spin-orbit coupling is progressively enhanced on increasing temperature, conflicting with theoretical prediction. This anomalous temperature dependence is explained by the interplay between the Kondo effect and the D'yakonov-Perel spin relaxation mechanism.

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Journal
Journal of Physics Condensed Matter
Published
2025-02-21
DOI
https://doi.org/10.1088/1361-648x/adb924
Primary Topic
Magnetic and transport properties of perovskites and related materials
Type
article
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Anomalous temperature dependence of spin–orbit coupling in Al2O3/SrTiO3 and Al2O3/KTaO3 heterostructures

Kuang‐Hong Gao, Tie Lin, Dingbang Zhou, Zhu Qin et al.
Journal of Physics Condensed Matter
Magnetic and transport properties of perovskites and related materials
article

Anomalous temperature dependence of spin–orbit coupling in Al2O3/SrTiO3 and Al2O3/KTaO3 heterostructures

Kuang‐Hong Gao, Tie Lin, Dingbang Zhou, Zhu Qin, Xiao Rong
article en

Abstract

Perovskite oxide-based heterostructures exhibit a range of exotic physical properties such as two-dimensional superconductivity, interface magnetism, tunable Kondo effect, and tunable spin-orbit coupling. Here, the magnetotransport properties of Al<sub>2</sub>O<sub>3</sub>/SrTiO<sub>3</sub>and Al<sub>2</sub>O<sub>3</sub>/KTaO<sub>3</sub>heterostructures are studied. Both Kondo effect and spin-orbit coupling-induced weak antilocalization (WAL) effect are observed at low temperatures. By analyzing the WAL curves, the spin relaxation time is extracted. Surprisingly, the extracted spin relaxation time unexpectedly decreases on increasing temperature in all samples. This indicates that the strength of the spin-orbit coupling is progressively enhanced on increasing temperature, conflicting with theoretical prediction. This anomalous temperature dependence is explained by the interplay between the Kondo effect and the D'yakonov-Perel spin relaxation mechanism.

Journal of Physics Condensed MatterVol. 37(15)
Tianjin University (CN), Tianjin Foreign Studies University (CN), Shanghai Institute of Technical Physics (CN), Tianjin haihe hospital (CN)
National Natural Science Foundation of China
Openalex Percentile: Top 98%
Magnetic and transport properties of perovskites and related materials
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Anomalous temperature dependence of spin–orbit coupling in Al<sub>2</sub>O<sub>3</sub>/SrTiO<sub>3</sub> and Al<sub>2</sub>O<sub>3</sub>/KTaO<sub>3</sub> heterostructures — Kuang‐Hong Gao, Tie Lin, et al. · Journal of Physics Condensed Matter (2025) | TGRS Research Map | TGRS