Mechanisms and Suppression of Quantum Dot Blinking

Abstract Colloidal quantum dots (QDs) have been awarded the 2023 Nobel Prize in Chemistry for their unique optoelectronic properties and great potential for applications. QD photoluminescence (PL) blinking research has made a significant contribution to the development of high quality QD materials and related applications. Almost all colloidal QDs are subject to PL blinking, a phenomenon in which the PL intensity of single QD randomly switches between different emission states. The blinking behavior disrupts the PL emission of QDs and hinders related QD‐based applications. Studies of QD blinking provide insight into the blinking mechanisms and contribute to the development of methods to suppress blinking. This review summarizes the significant advances in the understanding of PL blinking mechanisms and the development of suppression strategies since the first observation of PL blinking in single QDs. Specifically, it covers the Auger‐blinking mechanism, the band‐edge carrier blinking mechanism, the conversion of blinking types and their origins, the size dependence of blinking behavior, and various advanced blinking suppression strategies. Looking ahead, the integration of the advanced suppression strategies into various QD applications to unlock the full potential of colloidal QDs will be a key focus of future research.

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Publication Details

Journal
Laser & Photonics Review
Published
2025-02-19
DOI
https://doi.org/10.1002/lpor.202402269
Citations
10
Primary Topic
Quantum Dots Synthesis And Properties
Type
article
Field-Weighted Citation Impact
5.18

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article

Mechanisms and Suppression of Quantum Dot Blinking

Zhichun Yang, Ruiyun Chen, Chengbing Qin, Liantuan Xiao et al.
10 citations
Laser & Photonics Review
Quantum Dots Synthesis And Properties
5.18
article

Mechanisms and Suppression of Quantum Dot Blinking

Zhichun Yang, Ruiyun Chen, Chengbing Qin, Liantuan Xiao, Guofeng Zhang, Jianyong Hu, Changgang Yang, Suotang Jia, Jialu Li
article en
10 citations

Abstract

Abstract Colloidal quantum dots (QDs) have been awarded the 2023 Nobel Prize in Chemistry for their unique optoelectronic properties and great potential for applications. QD photoluminescence (PL) blinking research has made a significant contribution to the development of high quality QD materials and related applications. Almost all colloidal QDs are subject to PL blinking, a phenomenon in which the PL intensity of single QD randomly switches between different emission states. The blinking behavior disrupts the PL emission of QDs and hinders related QD‐based applications. Studies of QD blinking provide insight into the blinking mechanisms and contribute to the development of methods to suppress blinking. This review summarizes the significant advances in the understanding of PL blinking mechanisms and the development of suppression strategies since the first observation of PL blinking in single QDs. Specifically, it covers the Auger‐blinking mechanism, the band‐edge carrier blinking mechanism, the conversion of blinking types and their origins, the size dependence of blinking behavior, and various advanced blinking suppression strategies. Looking ahead, the integration of the advanced suppression strategies into various QD applications to unlock the full potential of colloidal QDs will be a key focus of future research.

Laser & Photonics ReviewVol. 19(9)
Shanxi University (CN), State Key Laboratory of Quantum Optics and Quantum Optics Devices
National Natural Science Foundation of China, China Postdoctoral Science Foundation, Natural Science Foundation of Shanxi Province, National Key Research and Development Program of China
Openalex Percentile: Top 4%
Quantum Dots Synthesis And Properties
5.18
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