Simultaneously Enhanced Mechanical Properties and Electromagnetic Interference Shielding Capabilities of Graphene Nanosheets Reinforced Magnesium Matrix Laminated Composite Using Accumulative Roll Bonding Process

In order to meet the demand for structural/functional integrated materials in the field of electromagnetic shielding, a graphene nanosheets (GNSs) reinforced magnesium matrix composite was fabricated using an electrophoretic deposition and subsequent accumulative roll bonding process (ARB). The microstructure, mechanical properties, and electromagnetic interference (EMI) shielding effectiveness (SE) of the GNSs/Mg composites were characterized systematically. The results showed that synergistic strengthening of the mechanical properties and EMI shielding performance of the composites was realized. The strengthening mechanisms for the mechanical and EMI shielding performance of the GNSs/Mg composites were analyzed thoroughly. After five passes of ARB, the ultimate tensile strength and elongation were 271.79 MPa and 12.9%, respectively. For the laminated structure, the strengthening is related to the thickness of the graphene layer, the dispersion, and the interfacial bonding with the metal matrix. In electromagnetic shielding aspects, after ARB-5, the SE is 93.36–105.15 dB. The introduction of well-organized multivariate multi-scale macro–micro interfaces increased the electromagnetic wave propagation paths and multiple reflection loss absorption in the internal propagation paths. Moreover, the addition of carbon nanomaterials led to an increase in the number of interfaces, which was conducive to the expansion of the internal reflection paths; carbon nanomaterials at the interfaces also improved the electromagnetic wave absorption.