Magnetoresistive reading of perpendicular magnetization in ferrimagnetic insulators enhanced through proximity coupling

Ferrimagnetic insulators with perpendicular magnetic anisotropy exhibit unique properties that offer potential for advanced spintronic devices. One of the challenges in exploiting these materials in spintronics lies in the efficient electrical detection of their magnetization. Herein we report the magnetoresistive detection of perpendicular magnetization in insulating ferrimagnetic garnets, enhanced through proximity coupling with an adjacent ultrathin ferromagnetic layer. We design and characterize a hybrid spin-valve device consisting of terbium iron garnet ($\mathrm{Tb}\mathrm{IG}$)$/\mathrm{Co}/\mathrm{Cu}/\mathrm{Tb}$-$\mathrm{Co}$ multilayers where $\mathrm{Tb}\mathrm{IG}$ and $\mathrm{Tb}$-$\mathrm{Co}$ are perpendicularly magnetized soft and hard layers, respectively, while $\mathrm{Co}$ is in-plane magnetized. We reveal through anomalous Hall effect and x-ray magnetic circular dichroism measurements that the interfacial exchange coupling between $\mathrm{Tb}\mathrm{IG}$ and $\mathrm{Co}$ induces a perpendicular magnetization component in the $\mathrm{Co}$ layer, which increases the magnetoresistance readout signal by more than 2 orders of magnitude---reaching 0.2%---compared with the reference system without the $\mathrm{Co}$ layer. A notable but less pronounced enhancement is observed in the $\mathrm{YIG}/\mathrm{Co}$-$\mathrm{Fe}$-$\mathrm{B}/\mathrm{Cu}/\mathrm{Tb}$-$\mathrm{Co}$ spin-valve device compared with the stack without the $\mathrm{Co}$-$\mathrm{Fe}$-$\mathrm{B}$ insertion, demonstrating the applicability of the approach to similar structures. Finally, we show that the magnetoresistive output signal can be effectively used to probe the multidomain state of $\mathrm{Tb}\mathrm{IG}$, opening a path for future insulating spintronic device applications.

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Publication Details

Journal
Physical Review Applied
Published
2025-02-18
DOI
https://doi.org/10.1103/physrevapplied.23.024042
Citations
1
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
1.25

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article

Magnetoresistive reading of perpendicular magnetization in ferrimagnetic insulators enhanced through proximity coupling

W. Janus, Can Onur Avci, Manuel Valvidares, Weibin Li
1 citations
Physical Review Applied
Magnetic properties of thin films
1.25
article

Magnetoresistive reading of perpendicular magnetization in ferrimagnetic insulators enhanced through proximity coupling

W. Janus, Can Onur Avci, Manuel Valvidares, Weibin Li
article en
1 citations

Abstract

Ferrimagnetic insulators with perpendicular magnetic anisotropy exhibit unique properties that offer potential for advanced spintronic devices. One of the challenges in exploiting these materials in spintronics lies in the efficient electrical detection of their magnetization. Herein we report the magnetoresistive detection of perpendicular magnetization in insulating ferrimagnetic garnets, enhanced through proximity coupling with an adjacent ultrathin ferromagnetic layer. We design and characterize a hybrid spin-valve device consisting of terbium iron garnet ($\mathrm{Tb}\mathrm{IG}$)$/\mathrm{Co}/\mathrm{Cu}/\mathrm{Tb}$-$\mathrm{Co}$ multilayers where $\mathrm{Tb}\mathrm{IG}$ and $\mathrm{Tb}$-$\mathrm{Co}$ are perpendicularly magnetized soft and hard layers, respectively, while $\mathrm{Co}$ is in-plane magnetized. We reveal through anomalous Hall effect and x-ray magnetic circular dichroism measurements that the interfacial exchange coupling between $\mathrm{Tb}\mathrm{IG}$ and $\mathrm{Co}$ induces a perpendicular magnetization component in the $\mathrm{Co}$ layer, which increases the magnetoresistance readout signal by more than 2 orders of magnitude---reaching 0.2%---compared with the reference system without the $\mathrm{Co}$ layer. A notable but less pronounced enhancement is observed in the $\mathrm{YIG}/\mathrm{Co}$-$\mathrm{Fe}$-$\mathrm{B}/\mathrm{Cu}/\mathrm{Tb}$-$\mathrm{Co}$ spin-valve device compared with the stack without the $\mathrm{Co}$-$\mathrm{Fe}$-$\mathrm{B}$ insertion, demonstrating the applicability of the approach to similar structures. Finally, we show that the magnetoresistive output signal can be effectively used to probe the multidomain state of $\mathrm{Tb}\mathrm{IG}$, opening a path for future insulating spintronic device applications.

Physical Review AppliedVol. 23(2)
ALBA Synchrotron (Spain) (ES), Institut de Ciència de Materials de Barcelona (ES)
Ministerio de Ciencia e Innovación, European Research Council, Horizon 2020
Openalex Percentile: Top 24%
Magnetic properties of thin films
1.25
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