Fluctuated lattice-driven charge density wave far above the condensation temperature in kagome superconductor KV3Sb5

The kagome material AV$_3$Sb$_5$ exhibits multiple exotic orders, including an unconventional charge density wave (CDW). Elucidating the underlying mechanism behind the CDW transition is crucial for unraveling the complex interactions among these phases. However, the driving force of the CDW remains a topic of debate due to the intertwined interactions among the system's various excitations. Here we investigated the CDW transition in KV$_3$Sb$_5$ by isolating the ultrafast electronic phase transition using time- and angleresolved photoemission spectroscopy. An ultrafast electronic phase transition was observed at a critical photoexcitation fluence, F$_c$, without reduction in CDW lattice-distortion-induced band folding. This folded band persisted up to 150 K under equilibrium heating, well above the CDW condensation temperature of T$_c$ = 78 K. Notably, the pump-induced band shifts at F$_c$ were comparable to those caused by thermal effects at T$_c$. These findings suggest that in KV$_3$Sb$_5$, a fluctuating lattice-driven in-plane CDW emerges above 150 K, with out-of-plane electronic correlations leading to the $2\times2 \times 2$ CDW near T$_c$, offering key insights into the interplay between the electronic and structural dynamics in AV$_3$Sb$_5$.

Authors

Institutions

Publication Details

Journal
Science Bulletin
Published
2025-02-18
DOI
https://doi.org/10.1016/j.scib.2025.02.018
Citations
4
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
5.03

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Fluctuated lattice-driven charge density wave far above the condensation temperature in kagome superconductor KV3Sb5

Jianzhe Liu, Yanfeng Guo, Zhihua Liu, Shaofeng Duan et al.
4 citations
Science Bulletin
Advanced Condensed Matter Physics
5.03
article

Fluctuated lattice-driven charge density wave far above the condensation temperature in kagome superconductor KV3Sb5

Jianzhe Liu, Yanfeng Guo, Zhihua Liu, Shaofeng Duan, Dong Qian, Xiangqi Liu, Shichong Wang, Lingxiao Gu, Wentao Zhang, Jian Huang, Haoran Liu, Wenxuan Yang
article en
4 citations

Abstract

The kagome material AV$_3$Sb$_5$ exhibits multiple exotic orders, including an unconventional charge density wave (CDW). Elucidating the underlying mechanism behind the CDW transition is crucial for unraveling the complex interactions among these phases. However, the driving force of the CDW remains a topic of debate due to the intertwined interactions among the system's various excitations. Here we investigated the CDW transition in KV$_3$Sb$_5$ by isolating the ultrafast electronic phase transition using time- and angleresolved photoemission spectroscopy. An ultrafast electronic phase transition was observed at a critical photoexcitation fluence, F$_c$, without reduction in CDW lattice-distortion-induced band folding. This folded band persisted up to 150 K under equilibrium heating, well above the CDW condensation temperature of T$_c$ = 78 K. Notably, the pump-induced band shifts at F$_c$ were comparable to those caused by thermal effects at T$_c$. These findings suggest that in KV$_3$Sb$_5$, a fluctuating lattice-driven in-plane CDW emerges above 150 K, with out-of-plane electronic correlations leading to the $2\times2 \times 2$ CDW near T$_c$, offering key insights into the interplay between the electronic and structural dynamics in AV$_3$Sb$_5$.

Science BulletinVol. 70(8)
Shanghai Jiao Tong University (CN), ShanghaiTech University (CN), Beijing National Laboratory for Molecular Sciences (CN), Ministry of Education (TW)
Natural Science Foundation of Shanghai, National Natural Science Foundation of China, China Postdoctoral Science Foundation, ShanghaiTech University, National Postdoctoral Program for Innovative Talents
Affordable and clean energy
Openalex Percentile: Top 6%
Advanced Condensed Matter Physics
5.03
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.