Fragile-to-strong glass transition in two-dimensional vortex liquids
The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mi>H</a:mi></a:math> applied perpendicularly to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:mi>X</b:mi><b:mi>Y</b:mi></b:mrow></b:math> model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength, a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile-to-strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.
Authors
- Ilaria Maccari (ORCID: https://orcid.org/0000-0003-2647-5242)
- C. Castellani (ORCID: https://orcid.org/0000-0002-4648-1693)
- Cristiano De Michele (ORCID: https://orcid.org/0000-0002-8367-0610)
- J. Lorenzana (ORCID: https://orcid.org/0000-0001-7426-2570)
- Lara Benfatto (ORCID: https://orcid.org/0000-0002-6091-3552)
Institutions
- ETH Zurich (CH)
- Sapienza University of Rome (IT)
Publication Details
- Journal
- Physical Review Research
- Published
- 2025-02-13
- DOI
- https://doi.org/10.1103/physrevresearch.7.013160
- Citations
- 1
- Primary Topic
- Material Dynamics and Properties
- Type
- article
- Field-Weighted Citation Impact
- 0.52
Funders
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung