Fragile-to-strong glass transition in two-dimensional vortex liquids

The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mi>H</a:mi></a:math> applied perpendicularly to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:mi>X</b:mi><b:mi>Y</b:mi></b:mrow></b:math> model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength, a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile-to-strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.

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Publication Details

Journal
Physical Review Research
Published
2025-02-13
DOI
https://doi.org/10.1103/physrevresearch.7.013160
Citations
1
Primary Topic
Material Dynamics and Properties
Type
article
Field-Weighted Citation Impact
0.52

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article

Fragile-to-strong glass transition in two-dimensional vortex liquids

Ilaria Maccari, C. Castellani, Cristiano De Michele, J. Lorenzana et al.
1 citations
Physical Review Research
Material Dynamics and Properties
0.52
article

Fragile-to-strong glass transition in two-dimensional vortex liquids

Ilaria Maccari, C. Castellani, Cristiano De Michele, J. Lorenzana, Lara Benfatto
article en
1 citations

Abstract

The fragile-to-strong glass transition is a fascinating phenomenon that still presents many theoretical and experimental challenges. A major one is how to tune the fragility of a glass-forming liquid. Here, we study a two-dimensional (2D) system composed of vortices in a superconducting film, which effectively behaves as a 2D glass-forming liquid. We show that the kinetic fragility in this system can be experimentally varied by tuning a single parameter: the external magnetic field <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mi>H</a:mi></a:math> applied perpendicularly to the film. This conclusion is supported by the direct comparison between the analysis of experimental measurements in an amorphous MoGe superconducting film and Monte Carlo simulations in a disordered <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mrow><b:mi>X</b:mi><b:mi>Y</b:mi></b:mrow></b:math> model, that captures the universality class of the two-step melting transition. We show that by increasing disorder strength, a fragile-to-strong transition is induced, in close similarity with the experimental findings in a magnetic field. Our numerical results shed light on the evolution of the dynamical heterogeneity from a fragile-to-strong glass, as due to the subtle interplay between caging effects arising from hexatic order and strong random pinning.

Physical Review ResearchVol. 7(1)
ETH Zurich (CH), Sapienza University of Rome (IT)
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
Openalex Percentile: Top 42%
Material Dynamics and Properties
0.52
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Fragile-to-strong glass transition in two-dimensional vortex liquids — Ilaria Maccari, C. Castellani, et al. · Physical Review Research (2025) | TGRS Research Map | TGRS