Sub‐MHz homogeneous linewidth in epitaxial Y <sub>2</sub> O <sub>3</sub> : Eu <sup>3+</sup> thin film on silicon
Thin films provide nanoscale confinement together with compatibility with photonic and microwave architectures, making them ideal candidates for chip-scale quantum devices. In this work, we propose a thin film fabrication approach yielding the epitaxial growth of Eu<sup>3+</sup> doped Y<sub>2</sub>O<sub>3</sub> on silicon. We combine two of the most prominent thin film deposition techniques: chemical vapor deposition (CVD) and molecular beam epitaxy (MBE). We report sub-megahertz optical homogeneous linewidths up to 8 K for the Eu<sup>3+</sup> dopants in the film, and lowest value of 270 kHz. This result constitutes a ten-fold improvement with respect to previous reports on the same material, opening promising perspectives for the development of scalable and compact quantum devices containing rare-earth ions.
Authors
- Alexey Tiranov (ORCID: https://orcid.org/0000-0003-0791-8730)
- Alban Ferrier (ORCID: https://orcid.org/0000-0002-9237-7635)
- Philippe Goldner (ORCID: https://orcid.org/0000-0001-8517-0911)
- Diana Serrano (ORCID: https://orcid.org/0000-0002-9478-3776)
- Tian Zhong (ORCID: https://orcid.org/0000-0003-3884-7453)
- Romain Bachelet (ORCID: https://orcid.org/0000-0002-2910-0449)
- Alexandre Tallaire (ORCID: https://orcid.org/0000-0002-0663-6662)
- N. Harada (ORCID: https://orcid.org/0000-0001-6947-080X)
- Anna Blin
Institutions
- Université Claude Bernard Lyon 1 (FR)
- École Centrale de Lyon (FR)
- Centre National de la Recherche Scientifique (FR)
- Chimie ParisTech - PSL (FR)
- Université Sorbonne Nouvelle (FR)
- Université Paris Sciences et Lettres (FR)
- Institut des Nanotechnologies de Lyon (FR)
- Sorbonne Université (FR)
- University of Chicago (US)
- Institut de Recherche de Chimie Paris (FR)
Publication Details
- Journal
- Nanophotonics
- Published
- 2025-02-13
- DOI
- https://doi.org/10.1515/nanoph-2024-0682
- Citations
- 2
- Primary Topic
- Silicon Nanostructures and Photoluminescence
- Type
- article
- Field-Weighted Citation Impact
- 1.04
Funders
- European Commission
- Agence Nationale de la Recherche