Diffusion transients in motility-induced phase separation

We numerically investigate normal diffusion in a two-dimensional athermal suspension of active particles undergoing motility-induced phase separation. The particles are modeled as achiral Janus disks with fixed self-propulsion speed and weakly fluctuating orientation. When plotted versus the overall suspension packing fraction, the relevant diffusion constant traces a hysteresis loop with sharp jumps in correspondence with the binodal and spinodal of the gaseous phase. No hysteresis loop is observed between the spinodal and binodal of the dense phase, as they appear to overlap. Moreover, even under steady-state phase separation, the particle displacement distributions exhibit non-Gaussian normal diffusion with transient fat (thin) tails in the presence (absence) of phase separation.

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Publication Details

Journal
Physical Review Research
Published
2025-02-12
DOI
https://doi.org/10.1103/physrevresearch.7.013153
Citations
10
Primary Topic
Micro and Nano Robotics
Type
article
Field-Weighted Citation Impact
12.58

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article

Diffusion transients in motility-induced phase separation

Shubhadip Nayak, Yuxin Zhou, Franco Nori, Yunyun Li et al.
10 citations
Physical Review Research
Micro and Nano Robotics
12.58
article

Diffusion transients in motility-induced phase separation

Shubhadip Nayak, Yuxin Zhou, Franco Nori, Yunyun Li, Poulami Bag, Fabio Marchesoni, Qingqing Yin, Pulak K. Ghosh
article en
10 citations

Abstract

We numerically investigate normal diffusion in a two-dimensional athermal suspension of active particles undergoing motility-induced phase separation. The particles are modeled as achiral Janus disks with fixed self-propulsion speed and weakly fluctuating orientation. When plotted versus the overall suspension packing fraction, the relevant diffusion constant traces a hysteresis loop with sharp jumps in correspondence with the binodal and spinodal of the gaseous phase. No hysteresis loop is observed between the spinodal and binodal of the dense phase, as they appear to overlap. Moreover, even under steady-state phase separation, the particle displacement distributions exhibit non-Gaussian normal diffusion with transient fat (thin) tails in the presence (absence) of phase separation.

Physical Review ResearchVol. 7(1)
Università di Camerino (IT), Tongji University (CN), Presidency University (IN), University of Michigan (US), RIKEN (JP), Quantum Chemistry Research Institute (JP)
University Grants Commission, National Natural Science Foundation of China, Science and Engineering Research Board, Japan Science and Technology Agency, RIKEN, Office of Naval Research
Life below water
Openalex Percentile: Top 1%
Micro and Nano Robotics
12.58
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