Near-Infrared Mobile Cloud OA-ICOS Sensor System for Atmospheric Carbon Dioxide Monitoring
Based on near-infrared off-axis integrated cavity output spectroscopy (OA-ICOS), a portable carbon dioxide (CO<sub>2</sub>) sensor system capable of atmosphere monitoring is proposed by targeting the CO<sub>2</sub> absorption lines at 2.004 μm. To address the comprehensive issues of complex light-adjustment structures, poor sealing, and slow gas replacement, an effective optimization scheme is introduced, combining fluid dynamics to produce a stable optical resonant cavity with an optical path length of 891 m and a physical length of 30 cm. The sensor system boasts a wide dynamic range of 0.011-800 parts per million (ppm), with a limit of detection (LoD) of 11 parts per billion (ppb) at an averaging time of 0.5 s. To address the issues of long monitoring time and cumbersome data supervision, a cloud monitoring system was developed based on a master control module, a cloud server, and a portable monitoring terminal. Field mobile monitoring of urban CO<sub>2</sub> was conducted over a large area in Changchun city, along with a 7-day fixed-point detection on the campus of Jilin University, verifying the reliability and application potential of the mobile CO<sub>2</sub> monitoring system in field applications.
Authors
- Kaiyuan Zheng (ORCID: https://orcid.org/0000-0002-5453-6770)
- Fang Song (ORCID: https://orcid.org/0000-0002-3921-1230)
- Zhiyong Chang (ORCID: https://orcid.org/0000-0002-2734-9267)
- Chuantao Zheng (ORCID: https://orcid.org/0000-0001-8008-466X)
- Lei Zhang (ORCID: https://orcid.org/0000-0003-3981-8101)
- Ying Hua
- Yishen Zhou
Institutions
- Hong Kong Polytechnic University (HK)
- Jilin University (CN)
- State Key Laboratory on Integrated Optoelectronics (CN)
- Jilin Medical University (CN)
Publication Details
- Journal
- Analytical Chemistry
- Published
- 2025-02-12
- DOI
- https://doi.org/10.1021/acs.analchem.4c05644
- Citations
- 8
- Primary Topic
- Atmospheric and Environmental Gas Dynamics
- Type
- article
- Field-Weighted Citation Impact
- 8.84
Funders
- National Natural Science Foundation of China
- People's Government of Jilin Province
- Education Department of Jilin Province
- National Key Research and Development Program of China