In-Situ Thermometry Reveals Fragmentation Behavior Based on Local Temperature in α-Olefin Polymerization Catalysts

Typical industrial olefin polymerization processes to produce both commodity and specialty polyolefin grades are mainly based on spherical, heterogeneous catalyst particles. During α-polymerization, heat from the exothermic reaction and pressure induced by the growing polymer chains on the catalyst particle lead to fragmentation, revealing active sites for further polymerization. To study these phenomena precisely and in-depth, we utilized a Nd-doped LaOCl-supported metallocene model system. This model catalyst can accurately display fluctuations in temperature with luminescence thermometry. During mild gas phase prepolymerization conditions, we observed a temperature difference of +43 °C and link this to the exothermicity of the ethylene polymerization reaction. In addition, the fragmentation behavior of the model catalyst was accurately monitored. The shell feature of the catalyst ruptured layer-by-layer, while the inner core fragmented via a bisectional fragmentation mechanism. We demonstrated that it is possible to probe the individual temperatures of multiple catalyst support particles within the field-of-view of the probe. This was correlated to structural changes and kinetics in an α-olefin polymerization catalyst. This powerful toolbox could be applied to different heterogeneous catalytic systems to correlate the temperature profile with morphological evolution.

Authors

Institutions

Publication Details

Journal
Journal of the American Chemical Society
Published
2025-02-10
DOI
https://doi.org/10.1021/jacs.4c11357
Citations
3
Primary Topic
Carbon dioxide utilization in catalysis
Type
article
Field-Weighted Citation Impact
2.11

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

In-Situ Thermometry Reveals Fragmentation Behavior Based on Local Temperature in α-Olefin Polymerization Catalysts

Florian Meirer, Joren M. Dorresteijn, Virginie Cirriez, Alexandre Welle et al.
3 citations
Journal of the American Chemical Society
Carbon dioxide utilization in catalysis
2.11
article

In-Situ Thermometry Reveals Fragmentation Behavior Based on Local Temperature in α-Olefin Polymerization Catalysts

Florian Meirer, Joren M. Dorresteijn, Virginie Cirriez, Alexandre Welle, Koen W. Bossers, Eelco T. C. Vogt, Bert Marc Weckhuysen, Thimo S. Jacobs, Bas J. P. Terlingen, Peter de Peinder, Yevkeni Wisse
article en
3 citations

Abstract

Typical industrial olefin polymerization processes to produce both commodity and specialty polyolefin grades are mainly based on spherical, heterogeneous catalyst particles. During α-polymerization, heat from the exothermic reaction and pressure induced by the growing polymer chains on the catalyst particle lead to fragmentation, revealing active sites for further polymerization. To study these phenomena precisely and in-depth, we utilized a Nd-doped LaOCl-supported metallocene model system. This model catalyst can accurately display fluctuations in temperature with luminescence thermometry. During mild gas phase prepolymerization conditions, we observed a temperature difference of +43 °C and link this to the exothermicity of the ethylene polymerization reaction. In addition, the fragmentation behavior of the model catalyst was accurately monitored. The shell feature of the catalyst ruptured layer-by-layer, while the inner core fragmented via a bisectional fragmentation mechanism. We demonstrated that it is possible to probe the individual temperatures of multiple catalyst support particles within the field-of-view of the probe. This was correlated to structural changes and kinetics in an α-olefin polymerization catalyst. This powerful toolbox could be applied to different heterogeneous catalytic systems to correlate the temperature profile with morphological evolution.

Journal of the American Chemical SocietyVol. 147(7)
Utrecht University (NL), Nanomaterials Research (United States) (US), Total (Belgium) (BE)
Universiteit Utrecht, Nederlandse Organisatie voor Wetenschappelijk Onderzoek, Total
Openalex Percentile: Top 18%
Carbon dioxide utilization in catalysis
2.11
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.