Control of Autler-Townes spectra by counter-rotating circularly polarized pulses

We theoretically investigate the resonant two-photon ionization of a hydrogen atom in the counter-rotating circularly polarized double-pulse sequences, by solving the time-dependent Schr"odinger equation. Due to the induced Rabi oscillations between the ground and excited states, the well-known Autler-Townes doublet is observed in the photoelectron spectra. More interestingly, our numerical results reveal an additional peak located between the Autler-Townes doublets, which originates from single-photon ionization from the excited state by the second pulse. By adjusting the laser intensity of the two pulses, the photoelectron yields of the three peaks can be sensitively modulated, under the control of completed Rabi cycles within the first pulse. In addition, our results show a potential of manipulating the photoemission anisotropy by both the laser intensity and the two-pulse time delay, through adjusting the competition of different partial waves generated by the two pulses.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-02-10
DOI
https://doi.org/10.1103/physreva.111.023106
Citations
2
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
2.49

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article

Control of Autler-Townes spectra by counter-rotating circularly polarized pulses

Yijie Liao, Yu Miao, Yueming Zhou, Xu Zhang et al.
2 citations
Physical review. A/Physical review, A
Laser-Matter Interactions and Applications
2.49
article

Control of Autler-Townes spectra by counter-rotating circularly polarized pulses

Yijie Liao, Yu Miao, Yueming Zhou, Xu Zhang, Peixiang Lu, Yuan Deng
article en
2 citations

Abstract

We theoretically investigate the resonant two-photon ionization of a hydrogen atom in the counter-rotating circularly polarized double-pulse sequences, by solving the time-dependent Schr\"odinger equation. Due to the induced Rabi oscillations between the ground and excited states, the well-known Autler-Townes doublet is observed in the photoelectron spectra. More interestingly, our numerical results reveal an additional peak located between the Autler-Townes doublets, which originates from single-photon ionization from the excited state by the second pulse. By adjusting the laser intensity of the two pulses, the photoelectron yields of the three peaks can be sensitively modulated, under the control of completed Rabi cycles within the first pulse. In addition, our results show a potential of manipulating the photoemission anisotropy by both the laser intensity and the two-pulse time delay, through adjusting the competition of different partial waves generated by the two pulses.

Physical review. A/Physical review, AVol. 111(2)
Wuhan National Laboratory for Optoelectronics (CN)
National Natural Science Foundation of China, Huazhong University of Science and Technology
Sustainable cities and communities
Openalex Percentile: Top 14%
Laser-Matter Interactions and Applications
2.49
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