Phonon heat transport and anisotropic tuning of quantum fluctuations in a frustrated honeycomb magnet

Honeycomb cobalt oxides containing $3d \mathrm{C}{\mathrm{o}}^{2+}$ ions might realize frustrated magnetism and novel quantum phases. Among candidate materials, $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ stands out for its distorted honeycomb lattice and significant in-plane anisotropy, motivating vector-field tuning inside the honeycomb plane. Here we use thermal transport down to the millikelvin regime to study twin-free crystals of $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ subject to in-plane vector fields. We find that the thermal conductivity $\ensuremath{\kappa}$ never exceeds the heat-transport capability of phonons, rendering its suppression primarily due to phonon scattering off magnetic excitations and/or domain boundaries. The system's field-driven quantum criticality manifests itself as an abundance of magnetic fluctuations hindering the heat transport, which further depends on the field direction in an intriguing manner. Our work establishes a powerful strategy of tuning magnetic quantum criticality with rotating fields and monitoring it with phonon heat transport.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-02-10
DOI
https://doi.org/10.1103/physrevb.111.085119
Citations
2
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
2.52

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article

Phonon heat transport and anisotropic tuning of quantum fluctuations in a frustrated honeycomb magnet

Xi Lin, Yuchen Gu, Yuan Li, Yue Chen et al.
2 citations
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
2.52
article

Phonon heat transport and anisotropic tuning of quantum fluctuations in a frustrated honeycomb magnet

Xi Lin, Yuchen Gu, Yuan Li, Yue Chen, Xintong Li, Haoran Fan
article en
2 citations

Abstract

Honeycomb cobalt oxides containing $3d \mathrm{C}{\mathrm{o}}^{2+}$ ions might realize frustrated magnetism and novel quantum phases. Among candidate materials, $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ stands out for its distorted honeycomb lattice and significant in-plane anisotropy, motivating vector-field tuning inside the honeycomb plane. Here we use thermal transport down to the millikelvin regime to study twin-free crystals of $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ subject to in-plane vector fields. We find that the thermal conductivity $\ensuremath{\kappa}$ never exceeds the heat-transport capability of phonons, rendering its suppression primarily due to phonon scattering off magnetic excitations and/or domain boundaries. The system's field-driven quantum criticality manifests itself as an abundance of magnetic fluctuations hindering the heat transport, which further depends on the field direction in an intriguing manner. Our work establishes a powerful strategy of tuning magnetic quantum criticality with rotating fields and monitoring it with phonon heat transport.

Physical review. B./Physical review. BVol. 111(8)
Chinese Academy of Sciences (CN), Peking University (CN), Hefei University (CN), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ), Beijing Academy of Quantum Information Sciences (CN)
National Science Foundation, National Key Research and Development Program of China
Openalex Percentile: Top 13%
Advanced Condensed Matter Physics
2.52
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