Phonon heat transport and anisotropic tuning of quantum fluctuations in a frustrated honeycomb magnet
Honeycomb cobalt oxides containing $3d \mathrm{C}{\mathrm{o}}^{2+}$ ions might realize frustrated magnetism and novel quantum phases. Among candidate materials, $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ stands out for its distorted honeycomb lattice and significant in-plane anisotropy, motivating vector-field tuning inside the honeycomb plane. Here we use thermal transport down to the millikelvin regime to study twin-free crystals of $\mathrm{N}{\mathrm{a}}_{3}\mathrm{C}{\mathrm{o}}_{2}\mathrm{Sb}{\mathrm{O}}_{6}$ subject to in-plane vector fields. We find that the thermal conductivity $\ensuremath{\kappa}$ never exceeds the heat-transport capability of phonons, rendering its suppression primarily due to phonon scattering off magnetic excitations and/or domain boundaries. The system's field-driven quantum criticality manifests itself as an abundance of magnetic fluctuations hindering the heat transport, which further depends on the field direction in an intriguing manner. Our work establishes a powerful strategy of tuning magnetic quantum criticality with rotating fields and monitoring it with phonon heat transport.
Authors
- Xi Lin (ORCID: https://orcid.org/0000-0002-9712-1882)
- Yuchen Gu (ORCID: https://orcid.org/0009-0002-2525-0527)
- Yuan Li (ORCID: https://orcid.org/0000-0002-2747-0649)
- Yue Chen (ORCID: https://orcid.org/0009-0008-5146-4522)
- Xintong Li (ORCID: https://orcid.org/0000-0001-8566-0558)
- Haoran Fan (ORCID: https://orcid.org/0009-0003-4625-2019)
Institutions
- Chinese Academy of Sciences (CN)
- Peking University (CN)
- Hefei University (CN)
- FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ)
- Beijing Academy of Quantum Information Sciences (CN)
Publication Details
- Journal
- Physical review. B./Physical review. B
- Published
- 2025-02-10
- DOI
- https://doi.org/10.1103/physrevb.111.085119
- Citations
- 2
- Primary Topic
- Advanced Condensed Matter Physics
- Type
- article
- Field-Weighted Citation Impact
- 2.52
Funders
- National Science Foundation
- National Key Research and Development Program of China