Real-space imaging of confined infrared surface plasmon polaritons on doped semiconductors covered with phase-change materials

Surface plasmon polaritons (SPPs) describe the excitation of photons coupled with free charge carriers at the interface of metals (visible) or doped semiconductors (infrared). While SPPs in the mid-infrared spectral range have been demonstrated in 2D materials such as graphene, their short propagation length combined with weak confinement in bulk materials has prevented real-space imaging of those SPPs. Here, we demonstrate real-space imaging of propagating SPPs on the doped semiconductors CdO and InAs with tunable plasma frequencies in the infrared via scattering-type scanning near-field optical microscopy. Adding a thin film of phase-change materials (PCMs) to these doped semiconductors increases the polariton confinement, leading to simplified SPP imaging and SPP resonator fabrication. We investigate optically written circular resonators of the plasmonic PCM In<sub>3</sub>SbTe<sub>2</sub> on CdO with near-field spectroscopy and Fabry-Perot resonators of the dielectric PCM Ge<sub>3</sub>Sb<sub>2</sub>Te<sub>6</sub> on InAs with far-field spectroscopy. Our work enables rapid prototyping of reconfigurable SPP resonators in mid-infrared.

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Publication Details

Journal
Science Advances
Published
2025-02-07
DOI
https://doi.org/10.1126/sciadv.adr6844
Citations
10
Primary Topic
Phase-change materials and chalcogenides
Type
article
Field-Weighted Citation Impact
5.18

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article

Real-space imaging of confined infrared surface plasmon polaritons on doped semiconductors covered with phase-change materials

Konstantin G. Wirth, Lukas Conrads, Dmitry N. Chigrin, Lena Jung et al.
10 citations
Science Advances
Phase-change materials and chalcogenides
5.18
article

Real-space imaging of confined infrared surface plasmon polaritons on doped semiconductors covered with phase-change materials

Konstantin G. Wirth, Lukas Conrads, Dmitry N. Chigrin, Lena Jung, Angela Cleri, Thomas Taubner, Matthias Wuttig, Andreas Heßler, Luis Schüler, Jon-Paul Maria
article en
10 citations

Abstract

Surface plasmon polaritons (SPPs) describe the excitation of photons coupled with free charge carriers at the interface of metals (visible) or doped semiconductors (infrared). While SPPs in the mid-infrared spectral range have been demonstrated in 2D materials such as graphene, their short propagation length combined with weak confinement in bulk materials has prevented real-space imaging of those SPPs. Here, we demonstrate real-space imaging of propagating SPPs on the doped semiconductors CdO and InAs with tunable plasma frequencies in the infrared via scattering-type scanning near-field optical microscopy. Adding a thin film of phase-change materials (PCMs) to these doped semiconductors increases the polariton confinement, leading to simplified SPP imaging and SPP resonator fabrication. We investigate optically written circular resonators of the plasmonic PCM In<sub>3</sub>SbTe<sub>2</sub> on CdO with near-field spectroscopy and Fabry-Perot resonators of the dielectric PCM Ge<sub>3</sub>Sb<sub>2</sub>Te<sub>6</sub> on InAs with far-field spectroscopy. Our work enables rapid prototyping of reconfigurable SPP resonators in mid-infrared.

Science AdvancesVol. 11(6)
Pennsylvania State University (US), RWTH Aachen University (DE)
Deutsche Forschungsgemeinschaft
Openalex Percentile: Top 4%
Phase-change materials and chalcogenides
5.18
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