Anomalous suppression of large-scale density fluctuations in classical and quantum spin liquids

Classical spin liquids (CSLs) are intriguing states of matter that do not exhibit long-range magnetic order and are characterized by an extensive ground-state degeneracy. Adding quantum fluctuations, which induce dynamics between these different classical ground states, can give rise to quantum spin liquids (QSLs). QSLs are highly entangled quantum phases of matter characterized by fascinating emergent properties, such as fractionalized excitations and topological order. One such exotic quantum liquid is the [Formula: see text] QSL, which can be regarded as a resonating valence bond (RVB) state formed from superpositions of dimer coverings of an underlying lattice. In this work, we unveil a hidden large-scale structural property of archetypal CSLs and QSLs known as hyperuniformity, i.e., normalized infinite-wavelength density fluctuations are completely suppressed in these systems. In particular, we first demonstrate that classical ensembles of close-packed dimers and their corresponding quantum RVB states are perfectly hyperuniform in general. Subsequently, we focus on a ruby-lattice spin liquid that was recently realized in a Rydberg-atom quantum simulator, and show that the QSL remains effectively hyperuniform even in the presence of a finite density of spinon and vison excitations, as long as the dimer constraint is still largely preserved. Moreover, we demonstrate that metrics based on the framework of hyperuniformity can be used to distinguish the QSL from other proximate quantum phases. These metrics can help identify potential QSL candidates, which can then be further analyzed using more advanced, computationally intensive quantum numerics to confirm their status as true QSLs.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2025-02-07
DOI
https://doi.org/10.1073/pnas.2416111122
Citations
8
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
10.06

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article

Anomalous suppression of large-scale density fluctuations in classical and quantum spin liquids

Duyu Chen, Salvatore Torquato, Yang Jiao, Rhine Samajdar
8 citations
Proceedings of the National Academy of Sciences
Advanced Condensed Matter Physics
10.06
article

Anomalous suppression of large-scale density fluctuations in classical and quantum spin liquids

Duyu Chen, Salvatore Torquato, Yang Jiao, Rhine Samajdar
article en
8 citations

Abstract

Classical spin liquids (CSLs) are intriguing states of matter that do not exhibit long-range magnetic order and are characterized by an extensive ground-state degeneracy. Adding quantum fluctuations, which induce dynamics between these different classical ground states, can give rise to quantum spin liquids (QSLs). QSLs are highly entangled quantum phases of matter characterized by fascinating emergent properties, such as fractionalized excitations and topological order. One such exotic quantum liquid is the [Formula: see text] QSL, which can be regarded as a resonating valence bond (RVB) state formed from superpositions of dimer coverings of an underlying lattice. In this work, we unveil a hidden large-scale structural property of archetypal CSLs and QSLs known as hyperuniformity, i.e., normalized infinite-wavelength density fluctuations are completely suppressed in these systems. In particular, we first demonstrate that classical ensembles of close-packed dimers and their corresponding quantum RVB states are perfectly hyperuniform in general. Subsequently, we focus on a ruby-lattice spin liquid that was recently realized in a Rydberg-atom quantum simulator, and show that the QSL remains effectively hyperuniform even in the presence of a finite density of spinon and vison excitations, as long as the dimer constraint is still largely preserved. Moreover, we demonstrate that metrics based on the framework of hyperuniformity can be used to distinguish the QSL from other proximate quantum phases. These metrics can help identify potential QSL candidates, which can then be further analyzed using more advanced, computationally intensive quantum numerics to confirm their status as true QSLs.

Proceedings of the National Academy of SciencesVol. 122(6)
Princeton University (US), University of California System (US), Center for Theoretical Physics (PL), Division of Materials Research (US), Arizona State University (US)
National Science Foundation, Aspen Center for Physics, Army Research Office
Openalex Percentile: Top 2%
Advanced Condensed Matter Physics
10.06
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