Theory of resonant x-ray scattering with ultrafast intense pulses

We present a time-dependent Schr"odinger equation approach within a nonrelativistic quantum electrodynamics framework to investigate resonant x-ray scattering driven by intense x-ray pulses. This method enables us to explore how coherent x-ray electron dynamics influence scattering signals from ${\mathrm{Ne}}^{+}$. We account for both resonance fluorescence and elastic scattering channels, while also considering competing photoionization and inner-shell decay processes. By computing the angular distribution and energy spectrum of scattered photons, we uncover interference effects between elastic scattering and resonance fluorescence pathways. Notably, this interference results in a small asymmetry in the energy spectrum. We discuss the experimental potential for detecting signatures of interference. Our findings demonstrate that the x-ray Rabi dynamics can be used to control scattering responses and provide insights into interference mechanisms and scattering efficiency in high-intensity x-ray regimes.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-02-05
DOI
https://doi.org/10.1103/physreva.111.023101
Citations
1
Primary Topic
Crystallography and Radiation Phenomena
Type
article
Field-Weighted Citation Impact
1.26

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article

Theory of resonant x-ray scattering with ultrafast intense pulses

Akilesh Venkatesh, Phay J. Ho
1 citations
Physical review. A/Physical review, A
Crystallography and Radiation Phenomena
1.26
article

Theory of resonant x-ray scattering with ultrafast intense pulses

Akilesh Venkatesh, Phay J. Ho
article en
1 citations

Abstract

We present a time-dependent Schr\"odinger equation approach within a nonrelativistic quantum electrodynamics framework to investigate resonant x-ray scattering driven by intense x-ray pulses. This method enables us to explore how coherent x-ray electron dynamics influence scattering signals from ${\mathrm{Ne}}^{+}$. We account for both resonance fluorescence and elastic scattering channels, while also considering competing photoionization and inner-shell decay processes. By computing the angular distribution and energy spectrum of scattered photons, we uncover interference effects between elastic scattering and resonance fluorescence pathways. Notably, this interference results in a small asymmetry in the energy spectrum. We discuss the experimental potential for detecting signatures of interference. Our findings demonstrate that the x-ray Rabi dynamics can be used to control scattering responses and provide insights into interference mechanisms and scattering efficiency in high-intensity x-ray regimes.

Physical review. A/Physical review, AVol. 111(2)
Argonne National Laboratory (US)
U.S. Department of Energy, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, Argonne National Laboratory
Climate action
Openalex Percentile: Top 25%
Crystallography and Radiation Phenomena
1.26
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Theory of resonant x-ray scattering with ultrafast intense pulses — Akilesh Venkatesh, Phay J. Ho · Physical review. A/Physical review, A (2025) | TGRS Research Map | TGRS