Theory of resonant x-ray scattering with ultrafast intense pulses
We present a time-dependent Schr"odinger equation approach within a nonrelativistic quantum electrodynamics framework to investigate resonant x-ray scattering driven by intense x-ray pulses. This method enables us to explore how coherent x-ray electron dynamics influence scattering signals from ${\mathrm{Ne}}^{+}$. We account for both resonance fluorescence and elastic scattering channels, while also considering competing photoionization and inner-shell decay processes. By computing the angular distribution and energy spectrum of scattered photons, we uncover interference effects between elastic scattering and resonance fluorescence pathways. Notably, this interference results in a small asymmetry in the energy spectrum. We discuss the experimental potential for detecting signatures of interference. Our findings demonstrate that the x-ray Rabi dynamics can be used to control scattering responses and provide insights into interference mechanisms and scattering efficiency in high-intensity x-ray regimes.
Authors
- Akilesh Venkatesh (ORCID: https://orcid.org/0000-0003-2141-4125)
- Phay J. Ho (ORCID: https://orcid.org/0000-0001-5214-2180)
Institutions
- Argonne National Laboratory (US)
Publication Details
- Journal
- Physical review. A/Physical review, A
- Published
- 2025-02-05
- DOI
- https://doi.org/10.1103/physreva.111.023101
- Citations
- 1
- Primary Topic
- Crystallography and Radiation Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 1.26
Funders
- U.S. Department of Energy
- Basic Energy Sciences
- Chemical Sciences, Geosciences, and Biosciences Division
- Argonne National Laboratory