Low temperature dependence of resistivity in obliquely sputter-deposited gold thin films

We report on the electrical resistivity at low temperature of Au thin films 400 nm thick deposited by DC magnetron sputtering using oblique angle deposition (OAD). The deposition angle α is gradually and systematically changed from 0° to 80°. A tilted and voided columnar structure is produced for deposition angles higher than 60°, whereas the lowest angles lead to a dense and compact structure with no clear cross-section morphology. Resistivity vs. temperature measurements reveal a typical metallic-like behavior in the range 7–300 K whatever the deposition angle. The latter gives rise to a significant increase of residual resistivity and temperature coefficient of resistance, and again for the most grazing angles, i.e. , α > 60°. The Bloch-Grüneisen model is assumed for understanding the evolution of electron-phonon interactions as a function of the deposition angle. This enhanced resistivity is connected to the structural defects and the porous architecture especially emphasized for glancing angles, and the strengthening of the electron-phonon coupling for high deposition angles. • Au thin films are sputtered by oblique angle deposition with an angle α = 0° to 80°. • A porous and tilted columnar architecture is produced for glancing deposition angles. • Resistivity vs. temperature is used to assess electron-phonon interactions. • The electron-phonon coupling strength enhances for high deposition angles.

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Publication Details

Journal
Surface and Coatings Technology
Published
2025-02-05
DOI
https://doi.org/10.1016/j.surfcoat.2025.131884
Citations
5
Primary Topic
Copper Interconnects and Reliability
Type
article
Field-Weighted Citation Impact
2.14

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article

Low temperature dependence of resistivity in obliquely sputter-deposited gold thin films

Stefania Oliveri, F. Sthal, Marina Raschetti, Nicolas Martin et al.
5 citations
Surface and Coatings Technology
Copper Interconnects and Reliability
2.14
article

Low temperature dependence of resistivity in obliquely sputter-deposited gold thin films

Stefania Oliveri, F. Sthal, Marina Raschetti, Nicolas Martin, E Tovar Martin, Joseph Gavoille, Jean-Marc Cote
article en
5 citations

Abstract

We report on the electrical resistivity at low temperature of Au thin films 400 nm thick deposited by DC magnetron sputtering using oblique angle deposition (OAD). The deposition angle α is gradually and systematically changed from 0° to 80°. A tilted and voided columnar structure is produced for deposition angles higher than 60°, whereas the lowest angles lead to a dense and compact structure with no clear cross-section morphology. Resistivity vs. temperature measurements reveal a typical metallic-like behavior in the range 7–300 K whatever the deposition angle. The latter gives rise to a significant increase of residual resistivity and temperature coefficient of resistance, and again for the most grazing angles, i.e. , α > 60°. The Bloch-Grüneisen model is assumed for understanding the evolution of electron-phonon interactions as a function of the deposition angle. This enhanced resistivity is connected to the structural defects and the porous architecture especially emphasized for glancing angles, and the strengthening of the electron-phonon coupling for high deposition angles. • Au thin films are sputtered by oblique angle deposition with an angle α = 0° to 80°. • A porous and tilted columnar architecture is produced for glancing deposition angles. • Resistivity vs. temperature is used to assess electron-phonon interactions. • The electron-phonon coupling strength enhances for high deposition angles.

Surface and Coatings TechnologyVol. 499
Centre National de la Recherche Scientifique (FR), Franche-Comté Électronique Mécanique Thermique et Optique - Sciences et Technologies (FR), École Normale Supérieure (BI), Laboratoire de Biologie et Pharmacologie Appliquée (FR), Université Marie et Louis Pasteur (FR)
Agence Nationale de la Recherche
Openalex Percentile: Top 14%
Copper Interconnects and Reliability
2.14
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