Nonequilibrium Binding Free Energy Simulations: Minimizing Dissipation

While nowadays approaches for equilibrium free energy estimation are well established, nonequilibrium simulations represent both an appealing computational opportunity and a challenge. This kind of simulations allows for a trivially parallel scheme, but at the same time the significant amount of irreversible work often generated during the steering process (either alchemical or physical) can hinder the convergence of free energy estimators. Here, we discuss in depth this issue for the protein-ligand binding free energy estimation carried out via physical paths. We found that the water model and the parametrization of the path collective variables have a remarkable impact on the convergence rate of the estimators (e.g., Crooks). Finally, we provide practical recipes to enhance the convergence speed and minimize dissipation.

Authors

Institutions

Publication Details

Journal
Journal of Chemical Theory and Computation
Published
2025-02-05
DOI
https://doi.org/10.1021/acs.jctc.4c01453
Citations
4
Primary Topic
Advanced Thermodynamics and Statistical Mechanics
Type
article
Field-Weighted Citation Impact
5.29

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Nonequilibrium Binding Free Energy Simulations: Minimizing Dissipation

Sergio Decherchi, Andrea Cavalli, Alessia Ghidini, Eleonora Serra
4 citations
Journal of Chemical Theory and Computation
Advanced Thermodynamics and Statistical Mechanics
5.29
article

Nonequilibrium Binding Free Energy Simulations: Minimizing Dissipation

Sergio Decherchi, Andrea Cavalli, Alessia Ghidini, Eleonora Serra
article en
4 citations

Abstract

While nowadays approaches for equilibrium free energy estimation are well established, nonequilibrium simulations represent both an appealing computational opportunity and a challenge. This kind of simulations allows for a trivially parallel scheme, but at the same time the significant amount of irreversible work often generated during the steering process (either alchemical or physical) can hinder the convergence of free energy estimators. Here, we discuss in depth this issue for the protein-ligand binding free energy estimation carried out via physical paths. We found that the water model and the parametrization of the path collective variables have a remarkable impact on the convergence rate of the estimators (e.g., Crooks). Finally, we provide practical recipes to enhance the convergence speed and minimize dissipation.

Journal of Chemical Theory and ComputationVol. 21(4)
Italian Institute of Technology (IT), École Polytechnique Fédérale de Lausanne (CH), University of Bologna (IT)
European Commission, University of California, San Francisco
Affordable and clean energy
Openalex Percentile: Top 5%
Advanced Thermodynamics and Statistical Mechanics
5.29
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.

Nonequilibrium Binding Free Energy Simulations: Minimizing Dissipation — Sergio Decherchi, Andrea Cavalli, et al. · Journal of Chemical Theory and Computation (2025) | TGRS Research Map | TGRS