Nonequilibrium Binding Free Energy Simulations: Minimizing Dissipation
While nowadays approaches for equilibrium free energy estimation are well established, nonequilibrium simulations represent both an appealing computational opportunity and a challenge. This kind of simulations allows for a trivially parallel scheme, but at the same time the significant amount of irreversible work often generated during the steering process (either alchemical or physical) can hinder the convergence of free energy estimators. Here, we discuss in depth this issue for the protein-ligand binding free energy estimation carried out via physical paths. We found that the water model and the parametrization of the path collective variables have a remarkable impact on the convergence rate of the estimators (e.g., Crooks). Finally, we provide practical recipes to enhance the convergence speed and minimize dissipation.
Authors
- Sergio Decherchi (ORCID: https://orcid.org/0000-0001-8371-2270)
- Andrea Cavalli (ORCID: https://orcid.org/0000-0002-6370-1176)
- Alessia Ghidini (ORCID: https://orcid.org/0000-0003-1063-7067)
- Eleonora Serra
Institutions
- Italian Institute of Technology (IT)
- École Polytechnique Fédérale de Lausanne (CH)
- University of Bologna (IT)
Publication Details
- Journal
- Journal of Chemical Theory and Computation
- Published
- 2025-02-05
- DOI
- https://doi.org/10.1021/acs.jctc.4c01453
- Citations
- 4
- Primary Topic
- Advanced Thermodynamics and Statistical Mechanics
- Type
- article
- Field-Weighted Citation Impact
- 5.29
Funders
- European Commission
- University of California, San Francisco