UV and NIR Dual-Band Photodetector Enabled by p-Type Perovskite and Semitransparent Microcavity
Narrowband photodetectors (NPDs) are essential for surveillance, photometry, and remote sensing. However, few studies have demonstrated multiple narrowband detection abilities within a single PD, particularly in the ultraviolet (UV) and near-infrared (NIR) regions, which are not directly recognized by the human eyes. In this work, we present a method for UV and NIR dual-band photodetection on the same device through integrating tandem-like perovskite/organic bulk-heterojunction (P-OBHJ) with a translucent microcavity. By leveraging the self-doping effect of perovskites, we fabricated p-type MAPbI3 films with the unbalanced electron–hole transport, enabling complete visible-light depletion upon bottom illumination. Meanwhile, NIR light passes through the entire perovskite layer to reach the OBHJ layers, ultimately resulting in a narrowband response to NIR light. Upon top illumination, the semitransparent microcavity selectively transmits only UV light, achieving narrowband UV detection. As a result, the optimized device exhibits the responsivity of 0.21 and 0.03 A/W with the corresponding shot-noise-limited specific detectivity reaching 4 × 1012 and 6 × 1011 Jones, at the peak wavelengths of 810 and 330 nm, respectively. Last, we showcase prototype applications of the dual-band PDs as heartbeat and solar UV intensity monitors, providing a novel strategy for the development of multifunctional NPD.
Authors
- Chenyang Han
- Zongmin Wang (ORCID: https://orcid.org/0000-0001-9204-5414)
- Qingshan Fan (ORCID: https://orcid.org/0000-0002-2993-0688)
- Keqiang Li (ORCID: https://orcid.org/0000-0001-9200-5906)
- Qiong Li (ORCID: https://orcid.org/0000-0003-1946-3673)
- Xiaodong Liu (ORCID: https://orcid.org/0000-0001-9639-1525)
- Hanqing Zhang (ORCID: https://orcid.org/0009-0006-9188-6776)
- Yu Zhou (ORCID: https://orcid.org/0000-0001-7624-2733)
- Zhenyu Wan (ORCID: https://orcid.org/0000-0001-6413-6765)
Institutions
- University of Electronic Science and Technology of China (CN)
- New York Genome Center (US)
Publication Details
- Journal
- ACS Photonics
- Published
- 2025-02-03
- DOI
- https://doi.org/10.1021/acsphotonics.4c02233
- Citations
- 5
- Primary Topic
- Perovskite Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 3.65
Funders
- Fundamental Research Funds for the Central Universities