UV and NIR Dual-Band Photodetector Enabled by p-Type Perovskite and Semitransparent Microcavity

Narrowband photodetectors (NPDs) are essential for surveillance, photometry, and remote sensing. However, few studies have demonstrated multiple narrowband detection abilities within a single PD, particularly in the ultraviolet (UV) and near-infrared (NIR) regions, which are not directly recognized by the human eyes. In this work, we present a method for UV and NIR dual-band photodetection on the same device through integrating tandem-like perovskite/organic bulk-heterojunction (P-OBHJ) with a translucent microcavity. By leveraging the self-doping effect of perovskites, we fabricated p-type MAPbI3 films with the unbalanced electron–hole transport, enabling complete visible-light depletion upon bottom illumination. Meanwhile, NIR light passes through the entire perovskite layer to reach the OBHJ layers, ultimately resulting in a narrowband response to NIR light. Upon top illumination, the semitransparent microcavity selectively transmits only UV light, achieving narrowband UV detection. As a result, the optimized device exhibits the responsivity of 0.21 and 0.03 A/W with the corresponding shot-noise-limited specific detectivity reaching 4 × 1012 and 6 × 1011 Jones, at the peak wavelengths of 810 and 330 nm, respectively. Last, we showcase prototype applications of the dual-band PDs as heartbeat and solar UV intensity monitors, providing a novel strategy for the development of multifunctional NPD.

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Publication Details

Journal
ACS Photonics
Published
2025-02-03
DOI
https://doi.org/10.1021/acsphotonics.4c02233
Citations
5
Primary Topic
Perovskite Materials and Applications
Type
article
Field-Weighted Citation Impact
3.65

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article

UV and NIR Dual-Band Photodetector Enabled by p-Type Perovskite and Semitransparent Microcavity

Chenyang Han, Zongmin Wang, Qingshan Fan, Keqiang Li et al.
5 citations
ACS Photonics
Perovskite Materials and Applications
3.65
article

UV and NIR Dual-Band Photodetector Enabled by p-Type Perovskite and Semitransparent Microcavity

Chenyang Han, Zongmin Wang, Qingshan Fan, Keqiang Li, Qiong Li, Xiaodong Liu, Hanqing Zhang, Yu Zhou, Zhenyu Wan
article en
5 citations

Abstract

Narrowband photodetectors (NPDs) are essential for surveillance, photometry, and remote sensing. However, few studies have demonstrated multiple narrowband detection abilities within a single PD, particularly in the ultraviolet (UV) and near-infrared (NIR) regions, which are not directly recognized by the human eyes. In this work, we present a method for UV and NIR dual-band photodetection on the same device through integrating tandem-like perovskite/organic bulk-heterojunction (P-OBHJ) with a translucent microcavity. By leveraging the self-doping effect of perovskites, we fabricated p-type MAPbI3 films with the unbalanced electron–hole transport, enabling complete visible-light depletion upon bottom illumination. Meanwhile, NIR light passes through the entire perovskite layer to reach the OBHJ layers, ultimately resulting in a narrowband response to NIR light. Upon top illumination, the semitransparent microcavity selectively transmits only UV light, achieving narrowband UV detection. As a result, the optimized device exhibits the responsivity of 0.21 and 0.03 A/W with the corresponding shot-noise-limited specific detectivity reaching 4 × 1012 and 6 × 1011 Jones, at the peak wavelengths of 810 and 330 nm, respectively. Last, we showcase prototype applications of the dual-band PDs as heartbeat and solar UV intensity monitors, providing a novel strategy for the development of multifunctional NPD.

ACS PhotonicsVol. 12(2)
University of Electronic Science and Technology of China (CN), New York Genome Center (US)
Fundamental Research Funds for the Central Universities
Openalex Percentile: Top 8%
Perovskite Materials and Applications
3.65
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