Detection of Atmospheric NO2 Using Scheimpflug DIAL with a Blue External Cavity Diode Laser Source

Nitrogen dioxide (NO2) is broadly acknowledged as one of the six key air pollutants, posing a significant threat to environmental stability and human health. The profile of atmospheric nitrogen dioxide is required for quantifying NO2 emissions from fossil fuel combustion and industry. In continuous-wave differential absorption lidar (CW-DIAL) systems, the laser sources employed are subject to the issues of varying output characteristics and poor instability. This study presents a CW-DIAL system for remote sensing of atmospheric NO2 that employs a compact grating-based external cavity diode laser (ECDL) and Scheimpflug imaging. The laser in this system utilizes a piezoelectric transducer (PZT) for precise wavelength tuning, emitting at 448.1 nm and 449.7 nm with an output power of 2.97 W and a narrow linewidth of 0.16 nm. Signal capturing was achieved through a Newtonian telescope with a diameter of 200 mm and a 45° inclined CCD image sensor, satisfying the Scheimpflug principle. A case study near road traffic was used to verify the feasibility of ECDL-DIAL, which took place from 1 October to 2 October 2023 over an industrial park. The system generates precise NO2 distribution maps with sub-50 m resolution over 3 km, updating every 10 min.