Thermal Stoner-Wohlfarth model for magnetodynamics of single domain nanoparticles: Implementation and validation

We present the thermal Stoner-Wohlfarth (tSW) model and apply it in the context of molecular dynamics simulations. The model is validated against an ensemble of immobilized, randomly oriented uniaxial particles (solid superparamagnet) and a classical dilute ferrofluid for different combinations of anisotropy strength and magnetic field/moment coupling, at a fixed temperature. We compare analytical and simulation results to quantify the viability of the tSW model in reproducing the equilibrium properties (with and without dipole-dipole interactions) and dynamic properties (without dipole-dipole interactions) of magnetic soft matter systems. We show that if the anisotropy of a particle is more than five times higher than the thermal fluctuations, the tSW model is applicable and efficient. This approach allows one to consider the interplay between N\'eel and Brownian relaxation, often neglected in the fixed point-dipole representation-based magnetic soft matter theoretical investigations.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-01-27
DOI
https://doi.org/10.1103/physrevb.111.014438
Citations
3
Primary Topic
Characterization and Applications of Magnetic Nanoparticles
Type
article
Field-Weighted Citation Impact
2.02

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article

Thermal Stoner-Wohlfarth model for magnetodynamics of single domain nanoparticles: Implementation and validation

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3 citations
Physical review. B./Physical review. B
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article

Thermal Stoner-Wohlfarth model for magnetodynamics of single domain nanoparticles: Implementation and validation

Pedro A. Sánchez, Claas Abert, Santiago Helbig, Deniz Mostarac, Dieter Suess, Sofia S. Kantorovich, Andrey Kuznetsov
article en
3 citations

Abstract

We present the thermal Stoner-Wohlfarth (tSW) model and apply it in the context of molecular dynamics simulations. The model is validated against an ensemble of immobilized, randomly oriented uniaxial particles (solid superparamagnet) and a classical dilute ferrofluid for different combinations of anisotropy strength and magnetic field/moment coupling, at a fixed temperature. We compare analytical and simulation results to quantify the viability of the tSW model in reproducing the equilibrium properties (with and without dipole-dipole interactions) and dynamic properties (without dipole-dipole interactions) of magnetic soft matter systems. We show that if the anisotropy of a particle is more than five times higher than the thermal fluctuations, the tSW model is applicable and efficient. This approach allows one to consider the interplay between N\'eel and Brownian relaxation, often neglected in the fixed point-dipole representation-based magnetic soft matter theoretical investigations.

Physical review. B./Physical review. BVol. 111(1)
University of Vienna (AT), Sapienza University of Rome (IT), Delft University of Technology (NL)
H2020 Marie Skłodowska-Curie Actions
Openalex Percentile: Top 16%
Characterization and Applications of Magnetic Nanoparticles
2.02
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