In Situ Study of the Temperature and Fluence Dependence of Yb2+ Luminescence in Yttrium Aluminum Garnet (YAG) Single Crystals
In this study, ion-beam-induced luminescence with 2 MeV H+ was used to excite YAG single crystals at different temperatures. Under several constant temperatures, the luminescence intensity of Yb2+ monotonically decreases with increasing fluence, eventually reaching approximately 35% of the initial intensity at a fluence of 3.5 × 1014 cm−2. The nonmonotonic evolution behavior of Yb2+ luminescence intensity with temperature can be effectively described by the intermediate-state model under consecutive temperature variations. The presence of an intermediate state may be the primary cause of the negative thermal quenching of Yb2+ luminescence. Yb2+ luminescence intensity decreased to 60% of the initial intensity when the temperature was continuously varied in the 100–300 K range, although the peak position remained rather stable. The luminescence of Yb2+ exhibits good radiation resistance and thermal stability in the experimental temperature range.
Authors
- Yingjie Song (ORCID: https://orcid.org/0000-0002-7224-2389)
- Hongtao Hu (ORCID: https://orcid.org/0000-0002-7323-2860)
- R.E. Chang
- Shasha Lv (ORCID: https://orcid.org/0000-0002-5219-7349)
- Guangfu Wang (ORCID: https://orcid.org/0000-0003-4065-1054)
- Menglin Qiu (ORCID: https://orcid.org/0009-0004-9590-5554)
Institutions
- Peking University (CN)
- Beijing Normal University (CN)
- Beijing Academy of Science and Technology (CN)
- State Key Laboratory of Nuclear Physics and Technology
Publication Details
- Journal
- Atoms
- Published
- 2025-01-27
- DOI
- https://doi.org/10.3390/atoms13020013
- Citations
- 2
- Primary Topic
- Luminescence Properties of Advanced Materials
- Type
- article
- Field-Weighted Citation Impact
- 1.04
Funders
- National Natural Science Foundation of China
- Natural Science Foundation for Young Scientists of Shanxi Province
- Young Scientists Fund