Triangular Lattice Magnet GdGa<sub>2</sub> with Short-Period Spin Cycloids and Possible Skyrmion Phases
The two-dimensional triangular lattice (TAL) is a model system of magnetic frustration and competing interactions, where skyrmion spin vortices can be induced by a vertical magnetic field $B$. We target the binary compound GdGa$_2$ with an undistorted TAL of Gd$^{3+}$ Heisenberg moments. At higher temperature ($T > 5$ K, $B = 0$, phase II), we reveal the cycloidal spin textures in GdGa$_2$ via resonant elastic X-ray scattering (REXS). Further, a transition with strong magneto-elastic response occurs when cooling into the zero-field ground state ($T < 5$ K, phase I). We also report the thermodynamic phase boundaries of $B$-induced magnetic A-phases, which are suppressed by an in-plane magnetic field and which have enhanced resistivity due to the partial opening of a charge gap. In analogy to Gd$_2$PdSi$_3$ and GdRu$_2$Si$_2$, these phases may represent a superposition of various cycloids, possibly a N\'eel skyrmion lattice. Our work lays the basis for further studies of the magnetic phase diagram of GdGa$_2$.
Authors
- Hironori Nakao (ORCID: https://orcid.org/0000-0003-4020-537X)
- T. Arima (ORCID: https://orcid.org/0000-0002-6959-0454)
- Masaki Gen (ORCID: https://orcid.org/0000-0003-1362-7323)
- Priya R. Baral (ORCID: https://orcid.org/0000-0002-9755-6165)
- Max Hirschberger (ORCID: https://orcid.org/0000-0002-1780-1619)
- N. D. Khanh (ORCID: https://orcid.org/0000-0002-4372-9278)
- Hajime Sagayama (ORCID: https://orcid.org/0000-0003-3816-9584)
- Yoshinori Tokura (ORCID: https://orcid.org/0000-0002-2732-4983)
- Yoshichika Ōnuki
Institutions
- High Energy Accelerator Research Organization (JP)
- RIKEN Center for Emergent Matter Science (JP)
- The University of Tokyo (JP)
Publication Details
- Journal
- Journal of the Physical Society of Japan
- Published
- 2025-01-27
- DOI
- https://doi.org/10.7566/jpsj.94.024705
- Citations
- 3
- Primary Topic
- Magnetic Properties of Alloys
- Type
- article
- Field-Weighted Citation Impact
- 1.28