Triangular Lattice Magnet GdGa<sub>2</sub> with Short-Period Spin Cycloids and Possible Skyrmion Phases

The two-dimensional triangular lattice (TAL) is a model system of magnetic frustration and competing interactions, where skyrmion spin vortices can be induced by a vertical magnetic field $B$. We target the binary compound GdGa$_2$ with an undistorted TAL of Gd$^{3+}$ Heisenberg moments. At higher temperature ($T > 5$ K, $B = 0$, phase II), we reveal the cycloidal spin textures in GdGa$_2$ via resonant elastic X-ray scattering (REXS). Further, a transition with strong magneto-elastic response occurs when cooling into the zero-field ground state ($T < 5$ K, phase I). We also report the thermodynamic phase boundaries of $B$-induced magnetic A-phases, which are suppressed by an in-plane magnetic field and which have enhanced resistivity due to the partial opening of a charge gap. In analogy to Gd$_2$PdSi$_3$ and GdRu$_2$Si$_2$, these phases may represent a superposition of various cycloids, possibly a N\'eel skyrmion lattice. Our work lays the basis for further studies of the magnetic phase diagram of GdGa$_2$.

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Publication Details

Journal
Journal of the Physical Society of Japan
Published
2025-01-27
DOI
https://doi.org/10.7566/jpsj.94.024705
Citations
3
Primary Topic
Magnetic Properties of Alloys
Type
article
Field-Weighted Citation Impact
1.28
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article

Triangular Lattice Magnet GdGa2 with Short-Period Spin Cycloids and Possible Skyrmion Phases

Hironori Nakao, T. Arima, Masaki Gen, Priya R. Baral et al.
3 citations
Journal of the Physical Society of Japan
Magnetic Properties of Alloys
1.28
article

Triangular Lattice Magnet GdGa2 with Short-Period Spin Cycloids and Possible Skyrmion Phases

Hironori Nakao, T. Arima, Masaki Gen, Priya R. Baral, Max Hirschberger, N. D. Khanh, Hajime Sagayama, Yoshinori Tokura, Yoshichika Ōnuki
article en
3 citations

Abstract

The two-dimensional triangular lattice (TAL) is a model system of magnetic frustration and competing interactions, where skyrmion spin vortices can be induced by a vertical magnetic field $B$. We target the binary compound GdGa$_2$ with an undistorted TAL of Gd$^{3+}$ Heisenberg moments. At higher temperature ($T > 5$ K, $B = 0$, phase II), we reveal the cycloidal spin textures in GdGa$_2$ via resonant elastic X-ray scattering (REXS). Further, a transition with strong magneto-elastic response occurs when cooling into the zero-field ground state ($T < 5$ K, phase I). We also report the thermodynamic phase boundaries of $B$-induced magnetic A-phases, which are suppressed by an in-plane magnetic field and which have enhanced resistivity due to the partial opening of a charge gap. In analogy to Gd$_2$PdSi$_3$ and GdRu$_2$Si$_2$, these phases may represent a superposition of various cycloids, possibly a N\'eel skyrmion lattice. Our work lays the basis for further studies of the magnetic phase diagram of GdGa$_2$.

Journal of the Physical Society of JapanVol. 94(2)
High Energy Accelerator Research Organization (JP), RIKEN Center for Emergent Matter Science (JP), The University of Tokyo (JP)
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Openalex Percentile: Top 23%
Magnetic Properties of Alloys
1.28
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