Determination of the thermal conductivity of nanowires based on the metal–insulator transition of VO2

We develop the theoretical foundation to determine the thermal conductivity of a single nanowire by using the optical contrast of the metallic and insulating domains of a VO2 nanowire excited with either a temperature difference or a laser beam. Considering the temperature dependence of the VO2 thermal conductivity, the heat flux and the temperature profile along a VO2 nanowire are obtained and used to derive explicit expressions for the position of the metal/insulator domain interface as a function of the thermal excitation. This relation determines the variations of the metallic and insulating domains’ lengths, which can be employed to retrieve the thermal conductivity of a single nanowire bonded to a VO2 one. Furthermore, the advantages and disadvantages of each thermal excitation are discussed along with the appearance of invariants driving the one-dimensional nonlinear heat conduction along VO2 nanowires.

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Publication Details

Journal
Journal of Applied Physics
Published
2025-01-10
DOI
https://doi.org/10.1063/5.0250479
Primary Topic
Transition Metal Oxide Nanomaterials
Type
article
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article

Determination of the thermal conductivity of nanowires based on the metal–insulator transition of VO2

José Ordoñez-Miranda, Laurent Belliard
Journal of Applied Physics
Transition Metal Oxide Nanomaterials
article

Determination of the thermal conductivity of nanowires based on the metal–insulator transition of VO2

José Ordoñez-Miranda, Laurent Belliard
article en

Abstract

We develop the theoretical foundation to determine the thermal conductivity of a single nanowire by using the optical contrast of the metallic and insulating domains of a VO2 nanowire excited with either a temperature difference or a laser beam. Considering the temperature dependence of the VO2 thermal conductivity, the heat flux and the temperature profile along a VO2 nanowire are obtained and used to derive explicit expressions for the position of the metal/insulator domain interface as a function of the thermal excitation. This relation determines the variations of the metallic and insulating domains’ lengths, which can be employed to retrieve the thermal conductivity of a single nanowire bonded to a VO2 one. Furthermore, the advantages and disadvantages of each thermal excitation are discussed along with the appearance of invariants driving the one-dimensional nonlinear heat conduction along VO2 nanowires.

Journal of Applied PhysicsVol. 137(2)
Centre National de la Recherche Scientifique (FR), Sorbonne Université (FR), Institut des NanoSciences de Paris (FR)
Affordable and clean energy
Openalex Percentile: Top 100%
Transition Metal Oxide Nanomaterials
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Determination of the thermal conductivity of nanowires based on the metal–insulator transition of VO2 — José Ordoñez-Miranda, Laurent Belliard · Journal of Applied Physics (2025) | TGRS Research Map | TGRS