Symmetries in three-dimensional photoelectron momentum spectroscopy as precursory methods for dichroic and enantiosensitive measurements
Three-dimensional photoelectron angular distributions (PADs) are measured from an atomic target ionized by ultrafast, elliptical fields of opposite handedness. Comparing these PADs to one another and to numeric simulations, a difficult to avoid systematic error in their orientation is identified and subsequently corrected by imposing the dichroic symmetry by which they are necessarily related. We show that this correction can be directly applied to molecular targets in the same fields. This paves the way for the measurement of enantiosensitive information, which has yet to be accessed experimentally.
Authors
- Van-Hung Hoang (ORCID: https://orcid.org/0000-0002-8538-7587)
- Michael Davino (ORCID: https://orcid.org/0000-0002-9463-9643)
- Andrés F. Ordóñez (ORCID: https://orcid.org/0000-0001-5274-4413)
- Tobias Saule (ORCID: https://orcid.org/0000-0002-2407-5176)
- George N. Gibson (ORCID: https://orcid.org/0000-0002-7537-2680)
- Edward McManus (ORCID: https://orcid.org/0000-0001-7755-9134)
- Carlos Trallero–Herrero (ORCID: https://orcid.org/0000-0002-9776-8125)
- Anh-Thu Le (ORCID: https://orcid.org/0000-0003-3577-4180)
- Phi-Hung Tran
Institutions
- Queen Mary University of London (GB)
- Kansas State University (US)
- Imperial College London (GB)
Publication Details
- Journal
- Physical Review Applied
- Published
- 2025-01-10
- DOI
- https://doi.org/10.1103/physrevapplied.23.014022
- Primary Topic
- Advanced Chemical Physics Studies
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Air Force Office of Scientific Research