Continuous-wave perovskite polariton lasers
Solution-processed semiconductor lasers are next-generation light sources for large-scale, bio-compatible and integrated photonics. However, overcoming their performance-cost trade-off to rival III-V laser functionalities is a long-standing challenge. Here, we demonstrate room-temperature continuous-wave perovskite polariton lasers exhibiting remarkably low thresholds of ~0.4 W cm<sup>-2</sup>, enabled by a variable single-crystal perovskite microcavity. The threshold outperforms state-of-the-art III-V lasers by ~30 times under optical pumping, and is exceptional among solution-processed lasers. The ultralow-threshold lasing arises from steady-state exciton-polariton condensation, a macroscopic quantum phenomenon akin to Bose-Einstein condensation. The steady-state condensation is attained by fine-tuning the cavity photon-exciton energy separation near the degeneracy point for strong light-matter interactions. These mechanisms enabled the initial demonstration of an indirectly injected perovskite laser chip powered by a gallium nitride light-emitting diode. Our findings create exciting avenues toward on-chip integration of solution-processed lasers, opening opportunities for lasing with ultralow energy consumption and unprecedented performance.
Authors
- Yaxiao Lian (ORCID: https://orcid.org/0009-0000-1938-3863)
- Yichen Yang (ORCID: https://orcid.org/0000-0002-3365-7178)
- Dawei Di (ORCID: https://orcid.org/0000-0003-0703-2809)
- Xuhui Cao
- Baodan Zhao (ORCID: https://orcid.org/0000-0002-4006-7061)
- Chen Zou (ORCID: https://orcid.org/0000-0001-9638-6363)
- Zixiang Wang (ORCID: https://orcid.org/0009-0002-1788-0668)
Institutions
- Zhejiang University (CN)
Publication Details
- Journal
- Science Advances
- Published
- 2025-01-10
- DOI
- https://doi.org/10.1126/sciadv.adr8826
- Citations
- 26
- Primary Topic
- Strong Light-Matter Interactions
- Type
- article
- Field-Weighted Citation Impact
- 32.42
Funders
- Zhejiang University