Continuous-wave perovskite polariton lasers

Solution-processed semiconductor lasers are next-generation light sources for large-scale, bio-compatible and integrated photonics. However, overcoming their performance-cost trade-off to rival III-V laser functionalities is a long-standing challenge. Here, we demonstrate room-temperature continuous-wave perovskite polariton lasers exhibiting remarkably low thresholds of ~0.4 W cm<sup>-2</sup>, enabled by a variable single-crystal perovskite microcavity. The threshold outperforms state-of-the-art III-V lasers by ~30 times under optical pumping, and is exceptional among solution-processed lasers. The ultralow-threshold lasing arises from steady-state exciton-polariton condensation, a macroscopic quantum phenomenon akin to Bose-Einstein condensation. The steady-state condensation is attained by fine-tuning the cavity photon-exciton energy separation near the degeneracy point for strong light-matter interactions. These mechanisms enabled the initial demonstration of an indirectly injected perovskite laser chip powered by a gallium nitride light-emitting diode. Our findings create exciting avenues toward on-chip integration of solution-processed lasers, opening opportunities for lasing with ultralow energy consumption and unprecedented performance.

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Publication Details

Journal
Science Advances
Published
2025-01-10
DOI
https://doi.org/10.1126/sciadv.adr8826
Citations
26
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
32.42

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article

Continuous-wave perovskite polariton lasers

Yaxiao Lian, Yichen Yang, Dawei Di, Xuhui Cao et al.
26 citations
Science Advances
Strong Light-Matter Interactions
32.42
article

Continuous-wave perovskite polariton lasers

Yaxiao Lian, Yichen Yang, Dawei Di, Xuhui Cao, Baodan Zhao, Chen Zou, Zixiang Wang
article en
26 citations

Abstract

Solution-processed semiconductor lasers are next-generation light sources for large-scale, bio-compatible and integrated photonics. However, overcoming their performance-cost trade-off to rival III-V laser functionalities is a long-standing challenge. Here, we demonstrate room-temperature continuous-wave perovskite polariton lasers exhibiting remarkably low thresholds of ~0.4 W cm<sup>-2</sup>, enabled by a variable single-crystal perovskite microcavity. The threshold outperforms state-of-the-art III-V lasers by ~30 times under optical pumping, and is exceptional among solution-processed lasers. The ultralow-threshold lasing arises from steady-state exciton-polariton condensation, a macroscopic quantum phenomenon akin to Bose-Einstein condensation. The steady-state condensation is attained by fine-tuning the cavity photon-exciton energy separation near the degeneracy point for strong light-matter interactions. These mechanisms enabled the initial demonstration of an indirectly injected perovskite laser chip powered by a gallium nitride light-emitting diode. Our findings create exciting avenues toward on-chip integration of solution-processed lasers, opening opportunities for lasing with ultralow energy consumption and unprecedented performance.

Science AdvancesVol. 11(2)
Zhejiang University (CN)
Zhejiang University
Affordable and clean energy
Openalex Percentile: Top 0%
Strong Light-Matter Interactions
32.42
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