Evidence for a metal–bosonic insulator–superconductor transition in compressed sulfur
The abrupt drop of resistance to zero at a critical temperature is a key signature of the current paradigm of the metal-superconductor transition. However, the emergence of an intermediate bosonic insulating state characterized by a resistance peak preceding the onset of the superconducting transition has challenged this traditional understanding. Notably, this phenomenon has been predominantly observed in disordered or chemically doped low-dimensional systems, raising intriguing questions about the generality of the effect and its underlying fundamental physics. Here, we present a systematic experimental study of compressed elemental sulfur, an undoped three-dimensional (3D) high-pressure superconductor, with detailed measurements of electrical resistance as a function of temperature, magnetic field, and current. The anomalous resistance peak observed in this 3D system is interpreted based on an empirical model of a metal-bosonic insulator-superconductor transition, potentially driven by vortex dynamics under magnetic field and energy dissipation processes. These findings offer a fresh platform for theoretical analysis of the decades-long enigmatic of the underlying mechanism of this phenomenon.
Authors
- Kui Wang (ORCID: https://orcid.org/0000-0002-9654-295X)
- Mi Zhou (ORCID: https://orcid.org/0000-0002-0697-5859)
- Qiushi Li (ORCID: https://orcid.org/0000-0003-1449-0568)
- Russell J. Hemley (ORCID: https://orcid.org/0000-0001-7398-8521)
- Yinqi Chen (ORCID: https://orcid.org/0000-0002-6885-3478)
- Hongbo Wang (ORCID: https://orcid.org/0000-0002-8031-5533)
- Guangtao Liu (ORCID: https://orcid.org/0000-0003-2332-115X)
- Hong Jian Zhao (ORCID: https://orcid.org/0000-0002-8921-2477)
- Yanming Ma (ORCID: https://orcid.org/0000-0003-3711-0011)
- Guangchen Ma
Institutions
- University of Illinois Urbana-Champaign (US)
- Jilin University (CN)
- University of Illinois Chicago (US)
- Jilin International Studies University (CN)
- State Key Laboratory of High Pressure and Superhard Materials (CN)
Publication Details
- Journal
- Proceedings of the National Academy of Sciences
- Published
- 2024-12-30
- DOI
- https://doi.org/10.1073/pnas.2420904122
- Citations
- 2
- Primary Topic
- High-pressure geophysics and materials
- Type
- article
- Field-Weighted Citation Impact
- 1.07
Funders
- National Science Foundation
- National Natural Science Foundation of China
- Chinese Academy of Sciences
- Division of Materials Research