Evidence for a metal–bosonic insulator–superconductor transition in compressed sulfur

The abrupt drop of resistance to zero at a critical temperature is a key signature of the current paradigm of the metal-superconductor transition. However, the emergence of an intermediate bosonic insulating state characterized by a resistance peak preceding the onset of the superconducting transition has challenged this traditional understanding. Notably, this phenomenon has been predominantly observed in disordered or chemically doped low-dimensional systems, raising intriguing questions about the generality of the effect and its underlying fundamental physics. Here, we present a systematic experimental study of compressed elemental sulfur, an undoped three-dimensional (3D) high-pressure superconductor, with detailed measurements of electrical resistance as a function of temperature, magnetic field, and current. The anomalous resistance peak observed in this 3D system is interpreted based on an empirical model of a metal-bosonic insulator-superconductor transition, potentially driven by vortex dynamics under magnetic field and energy dissipation processes. These findings offer a fresh platform for theoretical analysis of the decades-long enigmatic of the underlying mechanism of this phenomenon.

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Publication Details

Journal
Proceedings of the National Academy of Sciences
Published
2024-12-30
DOI
https://doi.org/10.1073/pnas.2420904122
Citations
2
Primary Topic
High-pressure geophysics and materials
Type
article
Field-Weighted Citation Impact
1.07

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article

Evidence for a metal–bosonic insulator–superconductor transition in compressed sulfur

Kui Wang, Mi Zhou, Qiushi Li, Russell J. Hemley et al.
2 citations
Proceedings of the National Academy of Sciences
High-pressure geophysics and materials
1.07
article

Evidence for a metal–bosonic insulator–superconductor transition in compressed sulfur

Kui Wang, Mi Zhou, Qiushi Li, Russell J. Hemley, Yinqi Chen, Hongbo Wang, Guangtao Liu, Hong Jian Zhao, Yanming Ma, Guangchen Ma
article en
2 citations

Abstract

The abrupt drop of resistance to zero at a critical temperature is a key signature of the current paradigm of the metal-superconductor transition. However, the emergence of an intermediate bosonic insulating state characterized by a resistance peak preceding the onset of the superconducting transition has challenged this traditional understanding. Notably, this phenomenon has been predominantly observed in disordered or chemically doped low-dimensional systems, raising intriguing questions about the generality of the effect and its underlying fundamental physics. Here, we present a systematic experimental study of compressed elemental sulfur, an undoped three-dimensional (3D) high-pressure superconductor, with detailed measurements of electrical resistance as a function of temperature, magnetic field, and current. The anomalous resistance peak observed in this 3D system is interpreted based on an empirical model of a metal-bosonic insulator-superconductor transition, potentially driven by vortex dynamics under magnetic field and energy dissipation processes. These findings offer a fresh platform for theoretical analysis of the decades-long enigmatic of the underlying mechanism of this phenomenon.

Proceedings of the National Academy of SciencesVol. 122(1)
University of Illinois Urbana-Champaign (US), Jilin University (CN), University of Illinois Chicago (US), Jilin International Studies University (CN), State Key Laboratory of High Pressure and Superhard Materials (CN)
National Science Foundation, National Natural Science Foundation of China, Chinese Academy of Sciences, Division of Materials Research
Affordable and clean energy
Openalex Percentile: Top 23%
High-pressure geophysics and materials
1.07
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