Unified Variational Approach Description of Ground-State Phases of the Two-Dimensional Electron Gas

The two-dimensional electron gas (2DEG) is a fundamental model, which is drawing increasing interest because of recent advances in experimental and theoretical studies of 2D materials. Current understanding of the ground state of the 2DEG relies on quantum Monte Carlo calculations, based on variational comparisons of different Ansätze for different phases. We use a single variational ansatz, a general backflow-type wave function using a message-passing neural quantum state architecture, for a unified description across the entire density range. The variational optimization consistently leads to lower ground-state energies than previous best results. Transition into a Wigner crystal (WC) phase occurs automatically at r_{s}=37±1, a density lower than currently believed. Between the liquid and WC phases, the same ansatz and variational search strongly suggest the existence of intermediate states in a broad range of densities, with enhanced short-range nematic spin correlations.

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Publication Details

Journal
Physical Review Letters
Published
2024-12-30
DOI
https://doi.org/10.1103/physrevlett.133.266504
Citations
14
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
1.64
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article

Unified Variational Approach Description of Ground-State Phases of the Two-Dimensional Electron Gas

Yixiao Chen, Ryan Levy, Conor Smith, Shiwei Zhang et al.
14 citations
Physical Review Letters
Electronic and Structural Properties of Oxides
1.64
article

Unified Variational Approach Description of Ground-State Phases of the Two-Dimensional Electron Gas

Yixiao Chen, Ryan Levy, Conor Smith, Shiwei Zhang, Miguel A. Morales, Yubo Yang
article en
14 citations

Abstract

The two-dimensional electron gas (2DEG) is a fundamental model, which is drawing increasing interest because of recent advances in experimental and theoretical studies of 2D materials. Current understanding of the ground state of the 2DEG relies on quantum Monte Carlo calculations, based on variational comparisons of different Ansätze for different phases. We use a single variational ansatz, a general backflow-type wave function using a message-passing neural quantum state architecture, for a unified description across the entire density range. The variational optimization consistently leads to lower ground-state energies than previous best results. Transition into a Wigner crystal (WC) phase occurs automatically at r_{s}=37±1, a density lower than currently believed. Between the liquid and WC phases, the same ansatz and variational search strongly suggest the existence of intermediate states in a broad range of densities, with enhanced short-range nematic spin correlations.

Physical Review LettersVol. 133(26)
Princeton University (US), Flatiron Health (United States) (US), Flatiron Institute (US)
Openalex Percentile: Top 12%
Electronic and Structural Properties of Oxides
1.64
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Unified Variational Approach Description of Ground-State Phases of the Two-Dimensional Electron Gas — Yixiao Chen, Ryan Levy, et al. · Physical Review Letters (2024) | TGRS Research Map | TGRS