Bias Tunable SnS<sub>2</sub>/ReSe<sub>2</sub> Tunneling Photodetector with High Responsivity and Fast Response Speed
2D photodetectors operating in photovoltaic mode exhibit a trade-off between response speed and photoresponsivity. This work presents a phototransistor based on SnS<sub>2</sub>/ReSe<sub>2</sub> heterojunction. Under negative bias, the energy band spike at the heterojunction interface impedes the carrier drifting so that the dark current is as low as 10<sup>-13</sup> A. The tunneling under positive bias significantly reduces the transmission time of photogenerated carriers, which enhances the responsivity and specific detectivity to 32.77 A W<sup>-1</sup> and 5.77 × 10<sup>11</sup> Jones, respectively. Under reverse bias, the enhanced built-in electric field strengthens the rapid separation of photogenerated carriers, which elevates a response speed to 10.5/24.1 µs and a 3 dB bandwidth to 54.8 kHz. The device also exhibits a broad spectral detection capability, extending from the near-ultraviolet to the near-infrared. Furthermore, this work also executed high-quality ASCII communication and high-resolution broadband single-pixel imaging, which demonstrates great promise for incorporation into future broadband optoelectronic systems.
Authors
- Xiao Han (ORCID: https://orcid.org/0000-0003-3141-4495)
- Shaoxi Wang (ORCID: https://orcid.org/0000-0002-0230-2059)
- Kexin Gao (ORCID: https://orcid.org/0009-0001-2395-8102)
- Lin Cheng (ORCID: https://orcid.org/0000-0002-3285-0187)
- Wei Li (ORCID: https://orcid.org/0000-0003-0824-9866)
- Yucheng Wang (ORCID: https://orcid.org/0000-0001-5746-0081)
- Ruijing Yang (ORCID: https://orcid.org/0000-0002-0480-9566)
- Tianle Yin
- Xuetao Gan
Institutions
- Northwestern Polytechnical University (CN)
- Ministry of Industry and Information Technology (CN)
Publication Details
- Journal
- Small
- Published
- 2024-12-26
- DOI
- https://doi.org/10.1002/smll.202408379
- Citations
- 15
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 1.76
Funders
- National Natural Science Foundation of China
- China Postdoctoral Science Foundation
- Key Research and Development Projects of Shaanxi Province